Atomic nuclei are finite quantum systems composed of two distinct types of fermion--protons and neutrons. In a manner similar to that of electrons orbiting in an atom, protons and neutrons in a nucleus form shell structures. In the case of stable, naturally occurring nuclei, large energy gaps exist between shells that fill completely when the proton or neutron number is equal to 2, 8, 20, 28, 50, 82 or 126 (ref. 1). Away from stability, however, these so-called 'magic numbers' are known to evolve in systems with a large imbalance of protons and neutrons. Although some of the standard shell closures can disappear, new ones are known to appear. Studies aiming to identify and understand such behaviour are of major importance in the field of experimental and theoretical nuclear physics. Here we report a spectroscopic study of the neutron-rich nucleus (54)Ca (a bound system composed of 20 protons and 34 neutrons) using proton knockout reactions involving fast radioactive projectiles. The results highlight the doubly magic nature of (54)Ca and provide direct experimental evidence for the onset of a sizable subshell closure at neutron number 34 in isotopes far from stability.

At the radioactive ion beam facility REX-ISOLDE, neutron-rich zinc isotopes were investigated using lowenergy Coulomb excitation. These experiments have resulted in B(E2, 2 74,76 Zn and the determination of the energy of the first excited 2 + 1 states in 78,80 Zn. The zinc isotopes were produced by high-energy proton-(A = 74, 76, 80) and neutron-(A = 78) induced fission of 238 U, combined with selective laser ionization and mass separation. The isobaric beam was postaccelerated by the REX linear accelerator and Coulomb excitation was induced on a thin secondary target, which was surrounded by the MINIBALL germanium detector array. In this work, it is shown how the selective laser ionization can be used to deal with the considerable isobaric beam contamination and how a reliable normalization of the experiment can be achieved. The results for zinc isotopes and the N = 50 isotones are compared to collective model predictions and state-of-the-art large-scale shell-model calculations, including a recent empirical residual interaction constructed to describe the present experimental data up to 2004 in this region of the nuclear chart.

3The general phenomenon of shell structure in atomic nuclei has been understood since the pioneering work of Goeppert-Mayer, Haxel, Jensen and Suess [1].They realized that the experimental evidence for nuclear magic numbers could be explained by introducing a strong spin-orbit interaction in the nuclear shell model potential.However, our detailed knowledge of nuclear forces and the mechanisms governing the structure of nuclei, in particular far from stability, is still incomplete. In nuclei with equal neutron and proton numbers (N = Z), the unique nature of the atomic nucleus as an object composed of two distinct types of fermions can be expressed as enhanced correlations arising between neutrons and protons occupying orbitals with the same quantum numbers. Such correlations have been predicted to favor a new type of nuclear superfluidity; isoscalar neutron-proton pairing [2][3][4][5][6], in addition to normal isovector pairing (see Fig. 1). Despite many experimental efforts these predictions have not been confirmed. Here, we report on the first observation of excited states in N = Z = 46 nucleus 92 Pd. Gamma rays emitted following the 58 Ni( 36 Ar,2n) 92 Pd fusionevaporation reaction were identified using a combination of state-of-the-art highresolution -ray, charged-particle and neutron detector systems. Our results reveal evidence for a spin-aligned, isoscalar neutronproton coupling scheme, different from the previous prediction [2][3][4][5][6]. We suggest that this coupling scheme replaces normal superfluidity (characterized by seniority coupling [7,8]) in the ground and low-lying excited states of the heaviest N = Z nuclei. The strong isoscalar neutron-proton correlations in these N = Z nuclei are predicted to have a considerable impact on their level structures, and to influence the dynamics of the stellar rapid proton capture nucleosynthesis process.For all known nuclei, including those residing along the N = Z line up to around mass 80, a detailed analysis of their properties such as binding energies [9] and the spectroscopy of the excited states [10] strongly suggests that normal isovector (T = 1) pairing is dominant at low excitation energies. On the other hand, there are long standing predictions for a change in the heavier N = Z nuclei from a nuclear superfluid dominated by isovector pairing to a structure where isoscalar (T = 0) neutron-proton (np) pairing has a major influence as the mass number increases towards the exotic doubly magic nucleus 100 Sn [2-6], the heaviest N = Z nucleus to be bound. N = Z nuclei with mass number > 90 can only be produced in the laboratory with very low The two-neutron (2n) evaporation reaction channel following formation of the 94 Pd compound nucleus, leading to 92 Pd, was very weakly populated with a relative yield of less than 10 −5 of the total fusion cross section. Gamma rays from decays of excited states in 92 Pd were identified by comparing γ-ray spectra in coincidence with two emitted neutrons and no charged particles with γ-ray spectra in coincidence with oth...

Expérience GANIL, VAMOS, EXOGAMThe lifetimes of the first excited 2+ states in 62Fe and 64Fe have been measured for the first time using the recoil-distance Doppler shift method after multinucleon transfer reactions in inverse kinematics. A sudden increase of collectivity from 62Fe to 64Fe is observed. The experimental results are compared with new largescale shell-model calculations and Hartree-Fock-Bogolyubov–based configuration-mixing calculations using the Gogny D1S interaction. The results give a deeper understanding of the mechanism leading to an onset of collectivity near 68Ni, which is compared with the situation in the so-called island of inversion around 32Mg

Background: Multinucleon transfer reactions (MNT) are a competitive tool to populate exotic neutron-rich nuclei in a wide region of nuclei, where other production methods have severe limitations or cannot be used at all. Purpose: Experimental information on the yields of MNT reactions in comparison with theoretical calculations are necessary to make predictions for the production of neutron-rich heavy nuclei. It is crucial to determine the fraction of MNT reaction products which are surviving neutron emission or fission at the high excitation energy after the nucleon exchange. Method: Multinucleon transfer reactions in 136 Xe + 238 U have been measured in a high-resolution γ -ray/particle coincidence experiment. The large solid-angle magnetic spectrometer PRISMA coupled to the high-resolution Advanced Gamma Tracking Array (AGATA) has been employed. Beamlike reaction products after multinucleon transfer in the Xe region were identified and selected with the PRISMA spectrometer. Coincident particles were tagged by multichannel plate detectors placed at the grazing angle of the targetlike recoils inside the scattering chamber. Results: Mass yields have been extracted and compared with calculations based on the GRAZING model for MNT reactions. Kinematic coincidences between the binary reaction products, i.e., beamlike and targetlike nuclei, were exploited to obtain population yields for nuclei in the actinide region and compared to x-ray yields measured by AGATA. Conclusions: No sizable yield of actinide nuclei beyond Z = 93 is found to perform nuclear structure investigations. In-beam γ -ray spectroscopy is feasible for few-neutron transfer channels in U and the −2p channel populating Th isotopes.

The neutron-rich lead isotopes, up to 216 Pb, have been studied for the first time, exploiting the fragmentation of a primary uranium beam at the FRS-RISING setup at GSI. The observed isomeric states exhibit electromagnetic transition strengths which deviate from state-of-the-art shell-model calculations. It is shown that their complete description demands the introduction of effective three-body interactions and two-body transition operators in the conventional neutron valence space beyond 208 Pb. The shell model is nowadays able to provide a comprehensive view of the atomic nucleus [1]. It is a many-body theoretical framework, successful in explaining various features of the structure of nuclei, based on the definition of a restricted valence space where a suitable Hamiltonian can be diagonalized. This effective interaction originates from realistic two-body nuclear forces based on phenomenological nucleon-nucleon potentials, renormalized to be adapted to the truncated model space. Although the renormalization process can be treated in a rigorous mathematical way, the appearance of effective terms is often neglected in calculations, as a common but incorrect practice. The presence and relevance of these effective forces is well known also in other fields of physics, as for example in condensed matter studies [2]. Indeed, effective three-body terms appear already at the lower perturbation order [3]: PRL 109, 162502 (2012) P H Y S I C A L

Neutron-rich isotopes around lead, beyond N=126, have been studied exploiting the fragmentation of an uranium primary beam at the FRS-RISING setup at GSI. For the first time β-decay half-lives of 219 Bi and 211,212,213 Tl isotopes have been derived. The half-lives have been extracted using a numerical simulation developed for experiments in high-background conditions. Comparison with state of the art models used in r-process calculations is given, showing a systematic underestimation of the experimental values, at variance from close-lying nuclei.

The low-lying structure of the neutron-rich nucleus (50)Ar has been investigated at the Radioactive Isotope Beam Factory using in-beam γ-ray spectroscopy with (9)Be((54)Ca,(50)Ar+γ)X, (9)Be((55)Sc,(50)Ar+γ)X, and (9)Be((56)Ti,(50)Ar+γ)X multinucleon removal reactions at ∼220  MeV/u. A γ-ray peak at 1178(18) keV is reported and assigned as the transition from the first 2(+) state to the 0(+) ground state. A weaker, tentative line at 1582(38) keV is suggested as the 4(1)(+)→2(1)(+) transition. The experimental results are compared to large-scale shell-model calculations performed in the sdpf model space using the SDPF-MU effective interaction with modifications based on recent experimental data for exotic calcium and potassium isotopes. The modified Hamiltonian provides a satisfactory description of the new experimental results for (50)Ar and, more generally, reproduces the energy systematics of low-lying states in neutron-rich Ar isotopes rather well. The shell-model calculations indicate that the N=32 subshell gap in (50)Ar is similar in magnitude to those in (52)Ca and (54)Ti and, notably, predict an N=34 subshell closure in (52)Ar that is larger than the one recently reported in (54)Ca.