Atomic nuclei are finite quantum systems composed of two distinct types of fermion--protons and neutrons. In a manner similar to that of electrons orbiting in an atom, protons and neutrons in a nucleus form shell structures. In the case of stable, naturally occurring nuclei, large energy gaps exist between shells that fill completely when the proton or neutron number is equal to 2, 8, 20, 28, 50, 82 or 126 (ref. 1). Away from stability, however, these so-called 'magic numbers' are known to evolve in systems with a large imbalance of protons and neutrons. Although some of the standard shell closures can disappear, new ones are known to appear. Studies aiming to identify and understand such behaviour are of major importance in the field of experimental and theoretical nuclear physics. Here we report a spectroscopic study of the neutron-rich nucleus (54)Ca (a bound system composed of 20 protons and 34 neutrons) using proton knockout reactions involving fast radioactive projectiles. The results highlight the doubly magic nature of (54)Ca and provide direct experimental evidence for the onset of a sizable subshell closure at neutron number 34 in isotopes far from stability.

Characterisation of the few doubly magic nuclei, known and predicted, provides a benchmark for our knowledge of the fundamental forces that drive the evolution of shell closures with proton-to-neutron asymme

Excited states in 38,40,42 Si nuclei have been studied via in-beam γ-ray spectroscopy with multinucleon removal reactions. Intense radioactive beams of 40 S and 44 S provided at the new facility of the RIKEN Radioactive Isotope Beam Factory enabled γ-γ coincidence measurements. A prominent γ line observed with an energy of 742 (8) 23.20.Lv, 27.40.+z, 29.38.Db Shell closures and collectivity are important properties that characterize the atomic nucleus. Interchange of their dominance along isotopic or isotonic chains has attracted much attention. The recent extension of the research frontier to nuclei far away from the valley of stability has revealed several new phenomena for neutronor proton-number dependent nuclear structure. For example, a weakening or even disappearance of shell closures occur in several neutron-rich nuclei at N = 8 [1][2][3] and N = 20 [4][5][6]. A well known example in the case of N = 20 is the so-called 'island of inversion ' [7] located around the neutron-rich nucleus 32 Mg. The low excitation energy of the first 2 + state E x (2 + 1 ) and large E2 transition probability [4][5][6] clearly indicate shell quenching in 32 Mg despite the fact that N = 20 is traditionally a magic number. The next magic number, N = 28, which appears due to the f 7/2 -f 5/2 spin-orbit splitting, has also been explored [8][9][10][11][12][13]. Weakening of the shell closure is seen by the decrease of the 2 With proton number Z = 14 and neutron number N = 28, the nuclear structure of 42 Si is of special interest. A simple but important question that arises is whether the weakening of the N = 28 shell closure continues, causing an enhancement of nuclear collectivity, or if shell stability is restored owing to a possible doubly magic structure. A study on 42 Si was made by a two-proton removal reaction experiment with radioactive 44 S beams at the NSCL [15]. The small two-proton removal cross sec-

The β-decay half-lives of 38 neutron-rich isotopes from 36 Kr to 43 Mo and 116,117 Tc are reported here for the first time. These results when compared to previous standard models indicate an overestimation in the predicted half-lives by a factor of two or more in the A ≈ 110 region. A revised model based on the second generation gross theory of β decay better predicts the measured half-lives and suggests a more rapid flow of the rapid neutron-capture process (r-matter flow) through this region than previously predicted.About half of the elements heavier than Fe are thought to be produced in rapid neutron-capture process (rprocess) nucleosynthesis, a sequence of neutron-capture and β-decay processes. Although the astronomical site and the mechanism of the r-process are not yet fully understood, it is generally agreed that the process must occur in environments with extreme neutron densities. The study of the elemental distribution along the r-process path requires sensitive β-decay related information such as β-decay half-lives, β-delayed neutron-emission probabilities, and nuclear masses. In particular, determination of the timescale that governs matter flow from the r-process "seeds" to the heavy nuclei, as well as the distribution in the r-process peaks, depends sensitively on decay half-lives [1,2].Isotopes with extreme neutron-to-proton ratios in the mass region A = 110 − 125 have attracted special attention since theoretical r-process yields are found to underestimate isotopic abundances observed in the predicted global abundances by an order of magnitude or more [1,3,4]. This discrepancy has been investigated using numerous mass formulae that differ mainly in the strength of the nuclear shell closures [5,6]. The results indicate that considerable improvements in the global abundances of the isotopes can be achieved by assuming a quenching of the N = 82 shell gap. The properties of most of these crucial r-process nuclei are, however, currently unknown due to their extremely low production yields in the laboratory.A number of experimental studies on nuclei around neutron-rich krypton to technetium have been performed to investigate the region of the r-process path near N = 82 [7][8][9]. In the current work, we report on a first systematic study of the β-decay properties of very exotic, neutron-rich 36 Kr to 43 Tc nuclides that contribute to the r-process.Decay spectroscopy of very neutron-rich nuclei around A = 110 was performed at the recently-commissioned RIBF facility at RIKEN. A secondary beam, comprised of a cocktail of neutron-rich nuclei, was produced by inflight fission of a 345-MeV/nucleon 238 U beam in a 550-mg/cm 2 Be target. The primary beam was produced by the RIKEN cyclotron accelerator complex with a typical intensity ∼ 0.3 pnA at the production target posi-

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Neutron-rich N=22, 24, 26 magnesium isotopes were studied via in-beam γ-ray spectroscopy at the RIKEN Radioactive Isotope Beam Factory following secondary fragmentation reactions on a carbon target at ≈200 MeV/nucleon. In the one- and two-proton removal channels from 39Al and 40Si beams, two distinct γ-ray transitions were observed in 38Mg, while in the one-proton removal reaction from 37Al a new transition was observed in addition to the known 2(1)(+)→0(g.s.)(+) decay. From the experimental systematics and comparison to theoretical predictions it is concluded that the transitions belong to the 2(1)(+)→0(g.s.)(+) and 4(1)(+)→2(1)(+) decays in 36Mg and 38Mg, respectively. For 34Mg, previously reported 2(1)(+) and 4(1)(+) level energies were remeasured. The deduced E(4(1)(+))/E(2(1)(+)) ratios for 34,36,38Mg of 3.14(5), 3.07(5), and 3.07(5) are almost identical and suggest the emergence of a large area of deformation extending from the N=20 to the N=28 shell quenching.

The lifetimes of the first excited states of the N = 30 isotones (50)Ca and (51)Sc have been determined using the Recoil Distance Doppler Shift method in combination with the CLARA-PRISMA spectrometers. This is the first time such a method is applied to measure lifetimes of neutron-rich nuclei populated via a multinucleon transfer reaction. This extends the lifetime knowledge beyond the f_{7/2} shell closure and allows us to derive the effective proton and neutron charges in the fp shell near the doubly magic nucleus (48)Ca, using large-scale, shell-model calculations. These results indicate an orbital dependence of the core polarization along the fp shell.