In situ x-ray diffraction studies of iron under shock conditions confirm unambiguously a phase change from the bcc (alpha) to hcp (epsilon) structure. Previous identification of this transition in shock-loaded iron has been inferred from the correlation between shock-wave-profile analyses and static high-pressure x-ray measurements. This correlation is intrinsically limited because dynamic loading can markedly affect the structural modifications of solids. The in situ measurements are consistent with a uniaxial collapse along the [001] direction and shuffling of alternate (110) planes of atoms, and are in good agreement with large-scale nonequilibrium molecular dynamics simulations.

The central goal of the National Ignition Facility (NIF) is demonstration of controlled thermonuclear ignition. The mainline ignition target is a low-Z, single-shell cryogenic capsule designed to have weakly nonlinear Rayleigh-Taylor growth of surface perturbations. Doubleshell targets are an alternative design concept that avoids the complexity of cryogenic preparation but has greater physics uncertainties associated with performance-degrading mix. A typical double-shell design involves a high-Z inner capsule filled with DT gas and supported within a low-Z ablator shell. The largest source of uncertainty for this target is the degree of highly evolved nonlinear mix on the inner surface of the high-Z shell. High Atwood numbers and feed-through of strong outer surface perturbation growth to the inner surface promote high levels of instability. The main challenge of the double-shell target designs is controlling the resulting nonlinear mix to levels that allow ignition to occur.Design and analysis of a suite of indirect-drive NIF double-shell targets with hohlraum temperatures of 200 eV and 250 eV are presented. Analysis of these targets includes assessment of two-dimensional radiation asymmetry as well as nonlinear mix. Twodimensional integrated hohlraum simulations indicate that the x-ray illumination can be adjusted to provide adequate symmetry control in hohlraums specially designed to have high laser-coupling efficiency [Suter et al., Phys. Plasmas 5, 2092(2000l. These simulations also reveal the need to diagnose and control localized 10-15 keV x-ray emission from the high-Z hohlraum wall because of strong absorption by the high-Z inner shell. Preliminary estimates of the degree of laser backscatter from an assortment of laser-plasma interactions suggest comparatively benign hohlraum conditions. Application of a variety of nonlinear mix models and phenomenological tools, including buoyancy-drag models, multimode simulations and fallline optimization, indicates a possibility of achieving ignition, i.e., fusion yields greater than 1 MJ. Planned experiments on the Omega laser to test current understanding of high-energy radiation flux asymmetry and mix-induced yield degradation in double-shell targets are described.

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A new method for shockless compression and acceleration of solid materials is presented. A plasma reservoir pressurized by a laser-driven shock unloads across a vacuum gap and piles up against an Al sample thus providing the drive. The rear surface velocity of the Al was measured with a line VISAR, and used to infer load histories. These peaked between approximately 0.14 and 0.5 Mbar with strain rates approximately 10(6)-10(8) s(-1). Detailed simulations suggest that apart from surface layers the samples can remain close to the room temperature isentrope. The experiments, analysis, and future prospects are discussed.

A dynamic transmission electron microscope (DTEM) has been designed and implemented to study structural dynamics in condensed matter systems. The DTEM is a conventional in situ transmission electron microscope (TEM) modified to drive material processes with a nanosecond laser, “pump” pulse and measure it shortly afterward with a 30-ns-long probe pulse of ∼107 electrons. An image with a resolution of <20nm may be obtained with a single pulse, largely eliminating the need to average multiple measurements and enabling the study of unique, irreversible events with nanosecond- and nanometer-scale resolution. Space charge effects, while unavoidable at such a high current, may be kept to reasonable levels by appropriate choices of operating parameters. Applications include the study of phase transformations and defect dynamics at length and time scales difficult to access with any other technique. This single-shot approach is complementary to stroboscopic TEM, which is capable of much higher temporal resolution but is restricted to the study of processes with a very high degree of repeatability.