The summer ozone pollution of Shandong province has become a severe problem in the period 2014–2018. Affected by the monsoon climate, the monthly average ozone concentrations in most areas were unimodal, with peaks in June, whereas in coastal areas the concentrations were bimodal, with the highest peak in May and the second highest peak in September. Using the empirical orthogonal function method, three main spatial distribution patterns were found. The most important pattern proved the influences of solar radiation, temperature, and industrial structure on ozone. Spatial clustering analysis of the ozone concentration showed Shandong divided into five units, including Peninsula Coastal area (PC), Lunan inland area (LN), Western Bohai area (WB), Luxi plain area (LX), and Luzhong mountain area (LZ). Influenced by air temperature and local circulation, coastal cities had lower daytime and higher nighttime ozone concentrations than inland. Correlation analysis suggested that ozone concentrations were significantly positively correlated with solar radiation. The VOCs from industries or other sources (e.g., traffic emission, petroleum processing, and chemical industries) had high positive correlations with ozone concentrations, whereas NOx emissions had significantly negatively correlation. This study provides a comprehensive understanding of ozone pollution and theoretical reference for regional management of ozone pollution in Shandong province.
Since the advent of photocatalytic degradation technology, it has brought new vitality to the environmental governance and the response to the energy crisis. Photocatalysts harvest optical energy to drive chemical reactions, which means people can use solar energy to complete some resource-consuming activities by photocatalysts, such as environmental governance. In recent years, researchers have tried to combine photocatalyst TiO 2 with building materials to purify urban air and obtained good results. One of the important functions of photocatalysts is to degrade organic pollutants in water through light energy, but this technology has not been reported in the practical application areas. To extend this technology to practical application areas, photocatalytic concrete for degrading pollutants in waters was proposed and demonstrated for the first time in this paper. The photocatalytic concrete proposed based on the K-g-C 3 N 4 shows a strong ability to degrade the organic dyes. According to the experiment results, the angle of light source plays an important role in the process of photocatalytic degradation, while waters with pH value of 6.5-8.5 hardly influenced the degradation of organic dyes. When the angle of light source is advantageous for photocatalytic concrete to absorb more visible light, more organic dyes will be degraded by photocatalytic concrete. The degradation rate of methylene blue could reach about 80% in ½ hour under desirable conditions and is satisfied compared with that of reported works. This study implicates that photocatalytic concrete can effectively degrade organic dyes in water. The influences of changes in the water environment hardly affect the degradation of organic pollutants, which means photocatalytic concrete can be widely used in green infrastructures to achieve urban sewage treatment.
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