We present the first report on the optical properties of dilute GaAS1-x
N
x
alloys (0<x<0.015). The layers have been grown by plasma-assisted metalorganic chemical vapor deposition (MOCVD). The grown layers show a systematic red shift of the band-edge luminescence with increasing N content. The assignement of the photoluminescence to band-edge transitions and not to isolated N-N pair emission is verified by the characteristics of the optical absorption.
A spectroscopic method, which enables characterization of a single isolated quantum dot and a quantum wave function interferometry, is applied to an exciton discrete excited state in an InGaAs quantum dot. Long coherence of zero-dimensional excitonic states made possible the observation of coherent population flopping in a 0D excitonic two-level system in a time-domain interferometric measurement. Corresponding energy splitting is also manifested in an energy-domain measurement.
Dye desorption and re-adsorption post treatments on electrochemically self-assembled nanoporous ZnO/eosinY hybrid thin films lead to a large improvement of the dye-sensitized photoelectrochemical performance, achieving an incident photon to current conversion efficiency up to 90%.
We first demonstrate a field-effect-transistor operation of dimetallofullerene La2@C80 with the icosahedral cage symmetry. The thin-film device showed an n-type behavior with a mobility of 1.1 x 10-4 cm2/V s at room temperature under high vacuum. Taking the nature of LUMO into account, the n-type behavior indicates an occurrence of carrier conduction through encapsulated La ions. The low mobility, suggesting an intermolecular hopping mechanism, is ascribed to the intrinsic and extrinsic reasons, which are discussed in the text.
Thymus- and activation-regulated chemokine (TARC/CCL17) is a lymphocyte-directed CC chemokine, which plays a role in the recruitment of CC chemokine receptor-4 positive T helper 2 (Th2) cells. In this study, we measured concentrations of TARC and Th2 cell-derived cytokines in bronchoalveolar lavage (BAL) fluid, as well as TARC concentrations in serum from patients with eosinophilic pneumonia and other interstitial lung diseases. TARC was significantly elevated in BAL fluids from patients with eosinophilic pneumonia (median, 240 pg/ml), whereas TARC was undetectable (< 7 pg/ml) in most cases of hypersensitivity pneumonitis, sarcoidosis, and idiopathic pulmonary fibrosis, as well as in healthy control subjects. Also, when present, quantities were less than 20 pg/ml. Elevated concentrations of interleukin (IL)-4, IL-5, and IL-13 were also detected in BAL fluid from patients with eosinophilic pneumonia. Interestingly, TARC concentrations in BAL fluids were closely correlated with the concentrations of IL-5 and IL-13. A serial examination showed that elevated TARC in BAL fluid rapidly fell to below detectable limits preceding decreases in IL-5 concentration and eosinophil percentage. Our results, in concordance with previous studies, demonstrate the potential activity of TARC for recruiting Th2 cells to the lungs and suggest a significant role for TARC in the pathogenesis of eosinophilic pneumonia.
We report the observation of spin relaxation of excitons in zero-dimensional semiconductor nanostructures. The spin relaxation is measured in InGaAs quantum disks by using a polarization dependent time-resolved photoluminescence method. The spin relaxation time in a zero-dimensional quantum disk is as long as 0.9 ns at 4 K, which is almost twice as long as the radiative recombination lifetime and is considerably longer than that in quantum wells. The temperature dependence of the spin relaxation time suggests the importance of exciton–acoustic phonon interaction.
Anisotropic magnetic-field evolution of the valence-band states in ideal Cd 1−x Mn x Te quantum wire structures have been studied theoretically by using multiband effective-mass method. The heavy-and light-hole bands show significant mixing owing to both the one-dimensional quantum confinement and the p-d exchange interaction. Because of the anisotropy of the initial quantization condition determined by the one-dimensional confinement, the Zeeman diagram of the valence bands exhibits anisotropic characteristics depending on the direction of the external magnetic field. According to the magnetic-field evolution of the valence-band states, the optical transition probability shows a dramatic change in the polarization.
We report on photon-spin controlled lasing oscillation in GaAs surface-emitting lasers at room temperature. We demonstrate experimentally that the partial electron-spin alignment, created by optically pumping the GaAs laser active media with circularly polarized pulses, drastically changes the polarization state of the lasing output, causing circularly polarized lasing emission. We discuss the laser polarization characteristics in relation to the measured electron-spin relaxation time.
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