Two-dimensional (2D) transition-metal dichalcogenides (TMDs) have drawn much attention due to their unique physical and chemical properties. Using TMDs as templates for the generation of 2D sandwich-like materials with remarkable properties still remains a great challenge due to their poor solvent processability. Herein, MoS2 -coupled sandwich-like conjugated microporous polymers (M-CMPs) with high specific surface area were successfully developed by using functionalized MoS2 nanosheets as template. As-prepared M-CMPs were further used as precursors for preparation of MoS2 -embedded nitrogen-doped porous carbon nanosheets, which were revealed as novel electrocatalysts for oxygen reduction reaction with mainly four-electron transfer mechanism and ultralow half-wave potential in comparison with commercial Pt/C catalyst. Our strategy to core-shelled sandwich-like hybrids paves a way for a new class of 2D hybrids for energy conversion and storage.
Although the most populous country in the world, China has limited palliative care programs. This article presents examples of three palliative care programs in China and encourages the program development in other Chinese hospitals.
Large-scale is a trend in person re-identi- fication (re-id). It is important that real-time search be performed in a large gallery. While previous methods mostly focus on discriminative learning, this paper makes the attempt in integrating deep learning and hashing into one framework to evaluate the efficiency and accuracy for large-scale person re-id. We integrate spatial information for discriminative visual representation by partitioning the pedestrian image into horizontal parts. Specifically, Part-based Deep Hashing (PDH) is proposed, in which batches of triplet samples are employed as the input of the deep hashing architecture. Each triplet sample contains two pedestrian images (or parts) with the same identity and one pedestrian image (or part) of the different identity. A triplet loss function is employed with a constraint that the Hamming distance of pedestrian images (or parts) with the same identity is smaller than ones with the different identity. In the experiment, we show that the proposed PDH method yields very competitive re-id accuracy on the large-scale Market-1501 and Market-1501+500K datasets.
EWOD was investigated from wetting to superwetting with six basic fluid systems. Each fluid system has developed special technologies for functional applications owing to the different interactions among solid, liquid and gas phases.
A series of trifluoromethyl pyridine derivatives containing 1,3,4-oxadiazole moiety was designed, synthesized and bio-assayed for their insecticidal activity. The result of bio-assays indicated the synthesized compounds exhibited good insecticidal activity against Mythimna separata and Plutella xylostella, most of the title compounds show 100% insecticidal activity at 500 mg L À1 and >80% activity at 250 mg L À1 against the two pests. Compounds E18 and E27 showed LC 50 values of 38.5 and 30.8 mg L À1 against Mythimna separata, respectively, which were close to that of avermectin (29.6 mg L À1 ); compounds E5, E6, E9, E10, E15, E25, E26, and E27 showed 100% activity at 250 mg L
À1, which were better than chlorpyrifos (87%). CoMFA and CoMSIA models with good predictability were proposed, which revealed the electron-withdrawing groups with an appropriate bulk at 2-and 4-positions of benzene ring could enhance insecticidal activity.
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.