The design, laboratory calibrations, and flight tests of a new optical imaging instrument, the two-dimensional stereo (2D-S) probe, are presented. Two orthogonal laser beams cross in the middle of the sample volume. Custom, high-speed, 128-photodiode linear arrays and electronics produce shadowgraph images with true 10-μm pixel resolution at aircraft speeds up to 250 m s−1. An overlap region is defined by the two laser beams, improving the sample volume boundaries and sizing of small (<∼100 μm) particles, compared to conventional optical array probes. The stereo views of particles in the overlap region can also improve determination of three-dimensional properties of some particles. Data collected by three research aircraft are examined and discussed. The 2D-S sees fine details of ice crystals and small water drops coexisting in mixed-phase cloud. Measurements in warm cumuli collected by the NCAR C-130 during the Rain in Cumulus over the Ocean (RICO) project provide a test bed to compare the 2D-S with 2D cloud (2D-C) and 260X probes. The 2D-S sees thousands of cloud drops <∼150 μm when the 2D-C and 260X probes see few or none. The data suggest that particle images and size distributions ranging from 25 to ∼150 μm and collected at airspeeds >100 m s−1 by the 2D-C and 260X probes are probably (erroneously) generated from out-of-focus particles. Development of the 2D-S is in its infancy, and much work needs to be done to quantify its performance and generate software to analyze data.

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to the Gleissberg minimum early in this century. However, the observed increase of about 20% is four times that expected based on the sunspot numbers.The observed high 44Ti and the inferred high GCR flux during the Gleissberg minimum suggest a much-weakened modulation of GCR during prolonged solar quiet periods. The heliosphere, during the 11vear solar cvcles. is divided into two hemispheres of dpposite polarity by a wavy heliospheric neutral sheet (HNS) whose inclination to the sun's rotational eauator increases from a few degrees at solar minimum to >70° at solar maximum and whose undulations also increase with solar activity (15). The HMF is relatively smooth during the solar minima. The enhanced GCR fluxes required for the higher production of 44Ti can be achieved if (i) the HNS becomes smooth and remains close to the helioequator; (ii) the HMF becomes weak, more regular, and orderlv; or (iii) the size of the , , . ,

[1] Oxalic acid is often the leading contributor to the total dicarboxylic acid mass in ambient organic aerosol particles. During the 2004 International Consortium for Atmospheric Research on Transport and Transformation (ICARTT) field campaign, nine inorganic ions (including SO 4 2À) and five organic acid ions (including oxalate) were measured on board the Center for Interdisciplinary Remotely Piloted Aircraft Studies (CIRPAS) Twin Otter research aircraft by a particle-into-liquid sampler (PILS) during flights over Ohio and surrounding areas. Five local atmospheric conditions were studied: (1) cloud-free air, (2) power plant plume in cloud-free air with precipitation from scattered clouds overhead, (3) power plant plume in cloud-free air, (4) power plant plume in cloud, and (5) clouds uninfluenced by local pollution sources. The aircraft sampled from two inlets: a counterflow virtual impactor (CVI) to isolate droplet residuals in clouds and a second inlet for sampling total aerosol. A strong correlation was observed between oxalate and SO 4 2À when sampling through both inlets in clouds. Predictions from a chemical cloud parcel model considering the aqueous-phase production of dicarboxylic acids and SO 4 2À show good agreement for the relative magnitude of SO 4 2À and oxalate growth for two scenarios: power plant plume in clouds and clouds uninfluenced by local pollution sources. The relative contributions of the two aqueous-phase routes responsible for oxalic acid formation were examined; the oxidation of glyoxylic acid was predicted to dominate over the decay of longer-chain dicarboxylic acids. Clear evidence is presented for aqueous-phase oxalic acid production as the primary mechanism for oxalic acid formation in ambient aerosols.

For 26 days in mid‐June and July 2000, a research group comprised of U.S. Navy, NASA, and university scientists conducted the Puerto Rico Dust Experiment (PRIDE). In this paper we give a brief overview of mean meteorological conditions during the study. We focus on our findings on African dust transported into the Caribbean utilizing a Navajo aircraft and AERONET Sun photometer data. During the study midvisible aerosol optical thickness (AOT) in Puerto Rico averaged 0.25, with a maximum >0.5 and with clean marine periods of ∼0.08. Dust AOTs near the coast of Africa (Cape Verde Islands and Dakar) averaged ∼0.4, 30% less than previous years. By analyzing dust vertical profiles in addition to supplemental meteorology and MPLNET lidar data we found that dust transport cannot be easily categorized into any particular conceptual model. Toward the end of the study period, the vertical distribution of dust was similar to the commonly assumed Saharan Air Layer (SAL) transport. During the early periods of the study, dust had the highest concentrations in the marine and convective boundary layers with only a weak dust layer in the SAL being present, a state usually associated with wintertime transport patterns. We corroborate the findings of Maring et al. [2003] that in most cases, there was an unexpected lack of vertical stratification of dust particle size. We systematically analyze processes that may impact dust vertical distribution and speculate that dust vertical distribution predominately influenced by flow patterns over Africa and differential advection coupled with fair weather cloud entrainment, mixing by easterly waves, and regional subsidence.