Abstract. On April 15 and 19, 1998, two intense dust storms were generated over the Gobi desert by springtime low-pressure systems descending from the northwest. The windblown dust was detected and its evolution followed by its yellow color on SeaWiFS satellite images, routine surface-based monitoring, and through serendipitous observations. The April 15 dust cloud was recirculating, and it was removed by a precipitating weather system over east Asia

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[1] We report summertime measurements of CO and O 3 obtained during 2001-2003 at the PICO-NARE mountaintop station in the Azores. Frequent events of elevated CO mixing ratios were observed. On the basis of backward trajectories arriving in the free troposphere and global simulations of biomass burning plumes, we attribute nearly all these events to North American pollution outflow and long-range transport of biomass burning emissions. There was a high degree of interannual variability in CO levels: median [CO] ranged from 65 ppbv in 2001 to 104 ppbv in 2003. The highest concentrations were associated with transport of Siberian fire emissions during summer 2003, when Siberian fire activity was unusually high. Ozone mixing ratios also increased (by up to $30 ppbv) during the fire events. These findings demonstrate the significant hemispheric scale impact that biomass burning events have on background CO and O 3 levels. O 3 enhancements of similar magnitude were also observed in North American pollution outflow. O 3 and CO were correlated during North American outflow events, with a slope averaging 1., ppbv/ppbv) when no fire impact was present. This slope is more than 80% larger than early 1990s observations made in the eastern United States and nearshore outflow region, even after accounting for declining U.S. CO emissions and for CO loss during transport to the Azores, and is not consistent with simple dilution of U.S. outflow with marine background air. We conclude that a significantly larger amount of O 3 production occurred in the air sampled during this study, and we suggest several potential reasons for this, each of which could imply potentially significant shortcomings in current estimates of the hemispheric impact of North American emissions on tropospheric ozone and should be evaluated in future studies.

[1] In this study, we present an aerosol data assimilation system destined for operational use at the Fleet Numerical Meteorological and Oceanographic Center (FNMOC). The system is an aerosol physics version of the Naval Research Laboratory (NRL) Atmospheric Variational Data Assimilation System (NAVDAS) that is already operational. The purpose of this new system, NAVDAS-Aerosol Optical Depth (NAVDAS-AOD) is to improve the NRL Aerosol Analysis and Prediction System (NAAPS)'s forecasting capability by assimilating observational data sources with NAAPS forecast fields. This will allow for not only improved aerosol forecasting but also for dramatically enhanced global scale research capabilities for the study of aerosol-meteorology interaction. NAVDAS-AOD assimilates a newly developed over-water Moderate-Resolution Imaging Spectroradiometers (MODIS) level 3 aerosol product with NAAPS. This paper is the second in a series which describes NRL's program to realistically monitor global aerosol distributions. Here we explain the reasons and procedures for constructing the over-water level 3 MODIS aerosol product, describe the theoretical basis for NAVDAS-AOD, and provide a thorough statistical error analysis for both the MODIS observations and the NAAPS model background fields that are critical to aerosol data assimilation. Using 5 months of analysis, our study shows that by carefully screening over-water satellite observations to ensure only the best quality data are used in the aerosol assimilation process, the NAVDAS-AOD can significantly improve the NAAPS global aerosol optical depth analysis as well as improve the aerosol forecast skill.

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For 26 days in mid‐June and July 2000, a research group comprised of U.S. Navy, NASA, and university scientists conducted the Puerto Rico Dust Experiment (PRIDE). In this paper we give a brief overview of mean meteorological conditions during the study. We focus on our findings on African dust transported into the Caribbean utilizing a Navajo aircraft and AERONET Sun photometer data. During the study midvisible aerosol optical thickness (AOT) in Puerto Rico averaged 0.25, with a maximum >0.5 and with clean marine periods of ∼0.08. Dust AOTs near the coast of Africa (Cape Verde Islands and Dakar) averaged ∼0.4, 30% less than previous years. By analyzing dust vertical profiles in addition to supplemental meteorology and MPLNET lidar data we found that dust transport cannot be easily categorized into any particular conceptual model. Toward the end of the study period, the vertical distribution of dust was similar to the commonly assumed Saharan Air Layer (SAL) transport. During the early periods of the study, dust had the highest concentrations in the marine and convective boundary layers with only a weak dust layer in the SAL being present, a state usually associated with wintertime transport patterns. We corroborate the findings of Maring et al. [2003] that in most cases, there was an unexpected lack of vertical stratification of dust particle size. We systematically analyze processes that may impact dust vertical distribution and speculate that dust vertical distribution predominately influenced by flow patterns over Africa and differential advection coupled with fair weather cloud entrainment, mixing by easterly waves, and regional subsidence.

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