Transition metal hybrid nanomaterials have attracted wide attention in the field of energy storage due to their rich redox activity and good conductivity and structural stability. In this work, low-crystalline...
A unique heteropolyoxotantalate (hetero-POTa) cluster
[P2O7Ta5O14]7– (P2Ta5) was first developed using pyrophosphate
as
a key to open the ultrastable skeleton of the classical Lindqvist-type
[Ta6O19]8– precursor. The
P2Ta5 cluster can serve as a general and flexible
secondary building unit to create a family of brand-new multidimensional
POTa architectures. This work not only promotes the limited structural
diversity of hetero-POTa but also provides a practical strategy for
new extended POTa architectures.
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