A differential absorption lidar has been built to measure CO2 concentration in the atmosphere. The transmitter is a pulsed single-frequency Ho:Tm:YLF laser at a 2.05-microm wavelength. A coherent heterodyne receiver was used to achieve sensitive detection, with the additional capability for wind profiling by a Doppler technique. Signal processing includes an algorithm for power measurement of a heterodyne signal. Results show a precision of the CO2 concentration measurement of 1%-2% 1sigma standard deviation over column lengths ranging from 1.2 to 2.8 km by an average of 1000 pulse pairs. A preliminary assessment of instrument sensitivity was made with an 8-h-long measurement set, along with correlative measurements with an in situ sensor, to determine that a CO2 trend could be detected.

A 2 microm wavelength, 90 mJ, 5 Hz pulsed Ho laser is described with wavelength control to precisely tune and lock the wavelength at a desired offset up to 2.9 GHz from the center of a CO(2) absorption line. Once detuned from the line center the laser wavelength is actively locked to keep the wavelength within 1.9 MHz standard deviation about the setpoint. This wavelength control allows optimization of the optical depth for a differential absorption lidar (DIAL) measuring atmospheric CO(2) concentrations. The laser transmitter has been coupled with a coherent heterodyne receiver for measurements of CO(2) concentration using aerosol backscatter; wind and aerosols are also measured with the same lidar and provide useful additional information on atmospheric structure. Range-resolved CO(2) measurements were made with <2.4% standard deviation using 500 m range bins and 6.7 min? (1000 pulse pairs) integration time. Measurement of a horizontal column showed a precision of the CO(2) concentration to <0.7% standard deviation using a 30 min? (4500 pulse pairs) integration time, and comparison with a collocated in situ sensor showed the DIAL to measure the same trend of a diurnal variation and to detect shorter time scale CO(2) perturbations. For vertical column measurements the lidar was setup at the WLEF tall tower site in Wisconsin to provide meteorological profiles and to compare the DIAL measurements with the in situ sensors distributed on the tower up to 396 m height. Assuming the DIAL column measurement extending from 153 m altitude to 1353 m altitude should agree with the tower in situ sensor at 396 m altitude, there was a 7.9 ppm rms difference between the DIAL and the in situ sensor using a 30 min? rolling average on the DIAL measurement.

The first airborne wind measurements of a pulsed, 2-mm solid-state, high-energy, wind-profiling lidar system for airborne measurements are presented. The laser pulse energy is the highest to date in an eye-safe airborne wind lidar system. This energy, the 10-Hz laser pulse rate, the 15-cm receiver diameter, and dualbalanced coherent detection together have the potential to provide much-improved lidar sensitivity to low aerosol backscatter levels compared to earlier airborne-pulsed coherent lidar wind systems. Problems with a laser-burned telescope secondary mirror prevented a full demonstration of the lidar's capability, but the hardware, algorithms, and software were nevertheless all validated. A lidar description, relevant theory, and preliminary results of flight measurements are presented.

A 2-µm backscatter lidar system has been developed by utilizing tunable pulsed laser and infrared phototransistor for the transmitter and the receiver, respectively. To validate the system, the 2-µm atmospheric backscatter profiles were compared to profiles obtained at 1 and 0.5 µm using avalanche photodiode and photomultiplier tube, respectively. Consequently, a methodology is proposed to compare the performance of different lidar systems operating at different wavelengths through various detection technologies. The methodology is based on extracting the system equivalent detectivity and comparing it to that of the detectors, as well as the ideal background detectivity. Besides, the 2-µm system capability for atmospheric CO 2 temporal profiling using the differential absorption lidar (DIAL) technique was demonstrated. This was achieved by tuning the laser at slightly different wavelengths around the CO 2 R22 absorption line in the 2.05-µm band. CO 2 temporal profiles were also compared to in situ measurements. Preliminary results indicated average mixing ratios close to 390 ppm in the atmospheric boundary layer with 3.0% precision. The development of this system is an initial step for developing a high-resolution, high-precision direct-detection atmospheric CO 2 DIAL system. A successful development of this system would be a valuable tool in obtaining and validating global atmospheric CO 2 measurements.

A single-frequency Ho:Tm:YLF laser, operating at an eye-safe wavelength of 2 mum, has been developed with tuning characteristics optimized for spectroscopy of absorption features. The laser frequency was stabilized to three different absorption lines of carbon dioxide by a wavelength modulation technique. Long-term frequency drift has been eliminated from the laser, and shorter-term jitter has been reduced to within 13.5 MHz of the absorption line center. This stabilized laser is an ideal injection seed source for a differential absorption lidar system for measurement of atmospheric gases.

Single-frequency lasing in monolithic crystals of holmium-thulium-doped YLF (Ho,Tm:YLF) is reported. A maximum single-frequency output power of 6 mW at a wavelength of 2.05 microm is demonstrated. Frequency tuning is also described.

We demonstrate wavelength control of a single-frequency diode-pumped Ho:Tm:YLF laser by referencing its wavelength to an absorption line of carbon dioxide. We accomplish this wavelength control by injection seeding with a cw Ho:Tm:YLF laser that can be tuned over or stabilized to carbon dioxide or water vapor lines. We show that the pulsed laser can be scanned precisely over an absorption line of carbon dioxide by scanning the injection seed laser wavelength. We locked the pulsed laser to within 18.5 MHz of the absorption line center by stabilizing the injection seed on the line center. The single-frequency pulsed output, intended for use as a transmitter for differential absorption lidar detection of atmospheric carbon dioxide and water vapor and for coherent detection of wind, is 100 mJ per pulse at a 5-Hz repetition rate.

High-energy 2-µm lasers have been incorporated in a breadboard coherent Doppler lidar to test component technologies and explore applications for remote sensing of the atmosphere. Design of the lidar is presented including aspects in the laser transmitter, receiver, photodetector, and signal processing. Sample data is presented on wind profiling and CO 2 concentration measurements.