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Since its last magmatic eruption in 1530 AD, La Soufrière andesitic volcano in Guadeloupe has displayed intense hydrothermal activity and six phreatic eruptive crises. Here we report on the first direct quantification of gas plume emissions from its summit vents, which gradually intensified during the past 20 years. Gas fluxes were determined in March 2006 and March 2012 by measuring the horizontal and vertical distributions of volcanic gas concentrations in the air-diluted plume and scaling to the speed of plume transport. Fluxes in 2006 combine realtime measurements of volcanic H 2 S concentrations and plume parameters with the composition of the hot (108.5°C) fumarolic fluid at exit. Fluxes in 2012 result from MultiGAS analysis of H 2 S, H 2 O, CO 2 , SO 2 and H 2 concentrations, combined with thermal imaging of the plume geometry and dynamics. Measurements were not only focused on the most active South crater (SC) vent, but also targeted Tarissan crater and other reactivating vents. We first demonstrate that all vents are fed by a common H 2 O-rich (97-98 mol%) fluid end-member, emitted almost unmodified at SC but affected by secondary shallow alterations at other vents. Daily fluxes in 2012 averaged 200 tons of H 2 O, 15 tons of CO 2 ,~4 tons of H 2 S and 1 ton of HCl, increased by a factor~3 compared to 2006. Even though modest, such fluxes make La Soufrière the second most important volcanic gas emitter in the Lesser Antilles arc, after Soufriere Hills of Montserrat. Taking account of other hydrothermal manifestations (hot springs and diffuse soil degassing), the summit fumarolic activity is shown to contribute most of the bulk volatile and heat budget of the volcano. The hydrothermal heat output (8 MW) exceeds by orders of magnitude the contemporaneous seismic energy release. Isotopic evidences support that La Soufrière hydrothermal emissions are sustained by a variable but continuous heat and gas supply from a magma reservoir confined at 6-7 km depth. By using petro-geochemical data for La Soufrière magma(s) and their dissolved volatile content, and assuming a magmatic derivation of sulfur, we estimate that the volcanic gas fluxes measured in 2012 could result from the underground release of magmatic gas exsolved from~1400 m 3 d −1 of basaltic melt feeding the system at depth. We recommend that fumarolic gas flux at La Soufrière becomes regularly measured in the future in order to carefully monitor the temporal evolution of that magmatic supply.

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Insights from long-term geochemical monitoring of halogenrich hydrothermal fluids. V illemant B. (1*) , K omorowski J C. (2,3) , Dessert C. (2,3) , M ichel A. (2) , C rispi O. (3) , H ammouya G. (3) , Beauducel F. (2,3) , De C habalier J.B. (2,3)

Abstract.Soufriere Hills fumaroles contained magmaderived volatiles before and during the eruption initiated in 1995 but also preserved a typical and quite steady hydrothermal coinposition. Chemical changes due to increased boiling and a greater input of oxidizing magmatic gas occurred only at Galway's Soufriere, the most active fumarolic field. Hydrothermal buffering of the fumaroles has been favoured by their remote location (!-2 km) froin the eruptive vents and by a preferential degassing of the uprising magma through intrusive conduits under the crater. High temperature (720øC) gas collected froin the extruding lava dome in Feb. 1996 was chemically and isotopically representative of the magmatic gas stream. Its coinposition allows assessment of average eruptive fluxes of H20, CO 2 and HCI which require the degassing of only 2.5-3 times more magma than erupted.