Nanostructures composed of dielectric, metallic or metalo-dielectric structures are receiving significant attention due to their unique capabilities to manipulate light for a wide range of functions such as spectral colors, anti-reflection and enhanced light-matter interaction. The optical properties of such nanostructures are determined not only by the shape and dimensions of the structures but also by their spatial arrangement. Here, we demonstrate the generation of vivid colors from nanostructures composed of spatially disordered metalo-dielectric (In/InP) nanopillar arrays. The nanopillars are formed by a single-step, ion-sputtering-assisted, self-assembly process that is inherently scalable and avoids complex patterning and deposition procedures. The In/InP nanopillar dimensions can be changed in a controlled manner by varying the sputter duration, resulting in reflective colors from pale blue to dark red. The fast Fourier transform (FFT) analysis of the distribution of the formed nanopillars shows that they are spatially disordered. The electromagnetic simulations combined with the optical measurements show that the reflectance spectra are strongly influenced by the pillar dimensions. While the specular and diffuse reflectance components are appreciable in all the nanopillar samples, the specular part dominates for the shorter nanopillars, thereby leading to a glossy effect. The simulation results show that the characteristic features in the observed specular and diffused reflectance spectra are determined by the modal and light-scattering properties of single pillars. While the work focuses on the In/InP system, the findings are relevant in a wider context of structural color generation from other types of metalo-dielectric nanopillar arrays.
Metasurfaces consisting of hybrid metal/dielectric nanostructures carry advantages of both material platforms. The hybrid structures can not only confine electromagnetic fields in subwavelength regions, but they may also lower the absorption losses. Such optical characteristics are difficult to realize in metamaterials with only metal or dielectric structures. Hybrid designs also expand the scope of material choices and the types of optical modes that can be excited in a metasurface, thereby allowing novel light matter interactions. Here, we present a metallo-dielectric hybrid metasurface design consisting of a high-index dielectric (silicon) nanodisk array on top of a metal layer (aluminum) separated by a buffer oxide (silica) layer. The dimensions of Si nanodisks are tuned to support anapole states and the period of the nanodisk array is designed to excite surface plasmon polariton (SPP) at the metal-buffer oxide interface. The physical dimensions of the Si nanodisk and the array periods are optimized to excite the anapole and the SPP at normal incidence of light in the visible-NIR (400-900 nm) wavelength range. Finite difference time domain (FDTD) simulations show that, when the nanodisk grating is placed at a specific height (∼200 nm) from the metal surface, the two modes strongly couple at zero detuning of the resonances. The strong coupling is evident from the avoided crossing of the modes observed in the reflectance spectra and in the spectral profile of light absorption inside the Si nanodisk. A vacuum Rabi splitting of up to ∼ 129 meV is achievable by optimizing the diameters of Si nanodisk and the nanodisk array grating period. The proposed metasurface design is promising to realize open cavity strongly coupled optical systems operating at room temperatures.
High index dielectric nanoresonators have gained prominence in nanophotonics due to lower losses compared to plasmonic systems and their ability to sustain both electric and magnetic resonances. The resonances can be engineered to create new types of optical states, such as bound-states in a continuum (BIC) and anapoles. In this work, we report on the optical properties of vertically stacked AlGaAs nanodisk Mie resonators. The nanodisks are designed to support an anapole state in the visible wavelength region (400–700 nm). The vertically stacked nanodisk resonators are fabricated from AlGaAs/GaAs multilayer samples with a fast and scalable patterning method using charged sphere colloidal lithography. Both measurements and finite difference time domain (FDTD) simulations of two and three stacked resonators show a sharp dip in the reflectance spectra at the anapole wavelength. For the 2 and 3 disk stacks the reflectance dip contrast at the anapole wavelength becomes very pronounced in the specular reflectance and is attributed to increased directional scattering due to an antenna effect. FDTD simulations show there is enhanced field confinement in all the disks at the anapole wavelength and the confined energy within the individual disks in the stack is at least 2–5 times greater compared to an isolated single nanodisk of the same dimension. Furthermore, the field confinement consistently increases with adding more disks in the stack. These vertically stacked AlGaAs nanodisk resonators can be a very exciting platform to engineer light matter interactions for linear and non-linear optical applications. The general principles of the fabrication method can be adapted to other wavelength ranges and can also be adapted for other III–V material combinations as well as for Si/SiO2.
The structural color from self-assembled metalo-dielectric (In/InP) nanopillars is shown to be polarization sensitive when the axial symmetry is broken. The characteristic dip in the reflection spectra due to resonant absorption is shifted by 90 nm as the polarization of incident light is altered from TE to TM at an incidence angle of 40°. We also show wafer-scale, mask-less fabrication of pillars that are tilted with respect to the substrate, a fast and cost effective method of creating the asymmetrical structures required for polarization sensitivity at normal incidence. A dip shift of 100 nm is observed for 40° tilted nanopillars of average height 380 nm, resulting in a smooth range of colors with changing polarization. FDTD simulations confirm the polarization dependent dip-shift in the resonant absorption wavelength. Furthermore, the field and intensity profiles obtained from the simulations indicate that the resonant absorption dips are due to HE1m-like modal excitations and their shift with respect to the incident angle and polarization leads to the change in perceived color from the tilted nanopillar system.
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