We probe the current-induced magnetic switching of insulating antiferromagnet/heavy metals systems, by electrical spin Hall magnetoresistance measurements and direct imaging, identifying a reversal occurring by domain wall (DW) motion. We observe switching of more than one third of the antiferromagnetic domains by the application of current pulses. Our data reveal two different magnetic switching mechanisms leading together to an efficient switching, namely the spin-current induced effective magnetic anisotropy variation and the action of the spin torque on the DWs. 2 MANUSCRIPTElectrical read-out and writing of the antiferromagnetic state is crucial to exploit the properties of antiferromagnets in future spintronic devices. Antiferromagnetic materials have the potential for ultrafast operation [1], with spin dynamics in the terahertz range, high packing density, due to the absence of stray magnetic fields, and an insensitivity to magnetic fields [2,3]. Furthermore, low-power operation is possible in antiferromagnetic insulators (AFM-Is) due to long spin diffusion lengths [4] and the theoretical prediction of superfluid spin transport [5].Recently, the electrical reading of the Néel order (n) orientation in AFM-Is was demonstrated via spin Hall magnetoresistance (SMR) [6-10], a magnetoresistive effect depending on the mutual orientation of the magnetic order and an interfacial spin accumulation μs. However, one of the main challenges faced by AFM spintronics is the reliable electrical writing of the orientation of n. One possible approach exploits staggered Néel spin orbit torques [11], creating an effective field of opposite sign on each magnetic sublattice. However, these torques rely on special material requirements, which has limited their application to the conducting AFMs CuMnAs and Mn2Au [12][13][14][15][16]. Another approach would be to use the non-staggered, antidamping-like torque exerted by a spin accumulation at the interface of a heavy metal and an AFM-I. A charge current in the heavy metal layer can generate a transverse spin current via the spin Hall effect, creating antidamping-like torques in the antiferromagnet.The possibility of such switching was demonstrated in NiO(001)/Pt and Pt/NiO(111)/Pt [17,18], but the mechanisms are still debated. One of the possible mechanisms relies on spin-current induced domain wall (DW) motion [19], predicting that DWs with opposite chirality are driven in opposite directions, thus excluding the electrical signature of the switching when DWs with opposite chirality are equally probable. A second mechanism [18], based on the coherent rotation of n, predicts a current threshold ten times larger than that found experimentally. A third mechanism, based on field-like torques acting on uncompensated interfacial spins, requires perfectly flat interfaces [17]. Currently, none of these provides a consistent explanation of the effect.In this work we realize reliable current-induced switching in epitaxial antiferromagnetic NiO/Pt bilayers. We show that the magnetic state of ...
Information transport and processing by pure magnonic spin currents in insulators is a promising alternative to conventional charge-current-driven spintronic devices. The absence of Joule heating and reduced spin wave damping in insulating ferromagnets have been suggested for implementing efficient logic devices. After the successful demonstration of a majority gate based on the superposition of spin waves, further components are required to perform complex logic operations. Here, we report on magnetization orientation-dependent spin current detection signals in collinear magnetic multilayers inspired by the functionality of a conventional spin valve. In Y3Fe5O12|CoO|Co, we find that the detection amplitude of spin currents emitted by ferromagnetic resonance spin pumping depends on the relative alignment of the Y3Fe5O12 and Co magnetization. This yields a spin valve-like behavior with an amplitude change of 120% in our systems. We demonstrate the reliability of the effect and identify its origin by both temperature-dependent and power-dependent measurements.
We measure the inverse spin Hall effect of CuIr thin films on yttrium iron garnet over a wide range of Ir concentrations (0.05 ⩽ x ⩽ 0.7). Spin currents are triggered through the spin Seebeck effect, either by a continuous (dc) temperature gradient or by ultrafast optical heating of the metal layer. The spin Hall current is detected by electrical contacts or measurement of the emitted terahertz radiation. With both approaches, we reveal the same Ir concentration dependence that follows a novel complex, nonmonotonous behavior as compared to previous studies. For small Ir concentrations a signal minimum is observed, whereas a pronounced maximum appears near the equiatomic composition. We identify this behavior as originating from the interplay of different spin Hall mechanisms as well as a concentration-dependent variation of the integrated spin current density in CuIr. The coinciding results obtained for dc and ultrafast stimuli provide further support that the spin Seebeck effect extends to terahertz frequencies, thus enabling a transfer of established spintronic measurement schemes into the terahertz regime. Our findings also show that the studied material allows for efficient spin-to-charge conversion even on ultrafast time scales.
In antiferromagnets, the efficient transport of spin-waves has until now only been observed in the insulating antiferromagnet hematite, where circularly (or a superposition of pairs of linearly) polarized spin-waves diffuse over long distances. Here, we report long-distance spin-transport in the antiferromagnetic orthoferrite YFeO3, where a different transport mechanism is enabled by the combined presence of the Dzyaloshinskii-Moriya interaction and externally applied fields. The magnon decay length is shown to exceed hundreds of nanometers, in line with resonance measurements that highlight the low magnetic damping. We observe a strong anisotropy in the magnon decay lengths that we can attribute to the role of the magnon group velocity in the transport of spin-waves in antiferromagnets. This unique mode of transport identified in YFeO3 opens up the possibility of a large and technologically relevant class of materials, i.e., canted antiferromagnets, for long-distance spin transport.
Understanding the electrical manipulation of antiferromagnetic order is a crucial aspect to enable the design of antiferromagnetic devices working at THz frequency. Focusing on collinear insulating antiferromagnetic NiO/Pt thin films as a materials platform, we identify the crystallographic orientation of the domains that can be switched by currents and quantify the Néel vector direction changes. We demonstrate electrical switching between different Tdomains by current pulses, finding that the Néel vector orientation in these domains is along [±1 ±1 3.8], different compared to the bulk <112 ̅ > directions. The final state of the Néel vector 𝒏 switching after current pulses 𝒋 along the [1 ± 1 0] directions is 𝒏 ∥ 𝒋. By comparing the observed Néel vector orientation and the strain in the thin films, assuming that this variation arises solely from magnetoelastic effects, we quantify the order of magnitude of the magnetoelastic coupling coefficient as 𝑏 0 + 2𝑏 1 = 3 × 10 7 J m 3 ⁄ . This information is key for the understanding of current-induced switching in antiferromagnets and for the design and use of such devices as active elements in spintronic devices.
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