Spintronics relies on the transport of spins, the intrinsic angular momentum of electrons, as an alternative to the transport of electron charge as in conventional electronics. The long-term goal of spintronics research is to develop spin-based, low-dissipation computing-technology devices. Recently, long-distance transport of a spin current was demonstrated across ferromagnetic insulators. However, antiferromagnetically ordered materials, the most common class of magnetic materials, have several crucial advantages over ferromagnetic systems for spintronics applications: antiferromagnets have no net magnetic moment, making them stable and impervious to external fields, and can be operated at terahertz-scale frequencies. Although the properties of antiferromagnets are desirable for spin transport, indirect observations of such transport indicate that spin transmission through antiferromagnets is limited to only a few nanometres. Here we demonstrate long-distance propagation of spin currents through a single crystal of the antiferromagnetic insulator haematite (α-FeO), the most common antiferromagnetic iron oxide, by exploiting the spin Hall effect for spin injection. We control the flow of spin current across a haematite-platinum interface-at which spins accumulate, generating the spin current-by tuning the antiferromagnetic resonance frequency using an external magnetic field. We find that this simple antiferromagnetic insulator conveys spin information parallel to the antiferromagnetic Néel order over distances of more than tens of micrometres. This mechanism transports spins as efficiently as the most promising complex ferromagnets. Our results pave the way to electrically tunable, ultrafast, low-power, antiferromagnetic-insulator-based spin-logic devices that operate without magnetic fields at room temperature.

A comprehensive mapping of the spin polarization of the electronic bands in ferroelectric α-GeTe(111) films has been performed using a time-of-flight momentum microscope equipped with an imaging spin filter that enables a simultaneous measurement of more than 10.000 data points (voxels). A Rashba type splitting of both surface and bulk bands with opposite spin helicity of the inner and outer Rashba bands is found revealing a complex spin texture at the Fermi energy. The switchable inner electric field of GeTe implies new functionalities for spintronic devices. The strong coupling of electron momentum and spin in low-dimensional structures allows an electrically controlled spin manipulation in spintronic devices [1-4], e.g. via the Rashba effect [5]. The Rashba effect has first been experimentally demonstrated in semiconductor heterostructures, where an electrical field perpendicular to the layered structure, i.e. perpendicular to the electron momentum, determines the electron spin orientation relative to its momentum [6-8]. An asymmetric interface structure causes the necessary inversion symmetry breaking and accounts for the special spin-splitting of electron states, the Rashba effect [5], the size of which can be tuned by the strength of the electrical field. For most semiconducting materials the Rashba effect causes only a quite small splitting of the order of 10 −2 ˚ A −1 and thus requires experiments at very low temperatures [9-11] and also implies large lateral dimensions for potential spintronic applications. A considerably larger splitting has been predicted theoretically [12] and was recently found experimentally for the surface states of GeTe(111) [13, 14]. GeTe is a ferroelectric semiconductor with a Curie temperature of 700 K. Thus, besides the interface induced Rashba splitting, the ferroelectric properties also imply a broken inversion symmetry within the bulk and thus would allow for the electrical tuning of the bulk Rashba splitting via switching the ferroelectric polarization [12, 15, 16]. This effect is of great interest for non-volatile spin orbitronics [10]. For GeTe a bulk Rashba splitting of 0.19Å19Å −1 has been predicted theoretically [12]. Experimentally, bulk-Rashba bands are rare and have only been found in the layered polar semiconductors BiTeCl and BiTeI [17-20] that, however, are not switchable. A characterization of the ferroelectric properties and a measurement of the spin polarization of the surface states of GeTe(111) at selected k-points has been performed previously by force microscopy [21, 22] and spin-resolved angular resolved photoemission spectroscopy, respectively [13]. A recent experimental and theoretical study revealed that at the Fermi level the hybridization of surface and bulk states causes surface-bulk resonant states resulting in unconventional spin topologies with chiral symmetry [14]. Here, we demonstrate the spin structure of surface and bulk bands of the GeTe(111) surface using the novel pho-toemission technique of spin-resolved time-of-flight momentum microsco...

We probe the current-induced magnetic switching of insulating antiferromagnet/heavy metals systems, by electrical spin Hall magnetoresistance measurements and direct imaging, identifying a reversal occurring by domain wall (DW) motion. We observe switching of more than one third of the antiferromagnetic domains by the application of current pulses. Our data reveal two different magnetic switching mechanisms leading together to an efficient switching, namely the spin-current induced effective magnetic anisotropy variation and the action of the spin torque on the DWs. 2 MANUSCRIPTElectrical read-out and writing of the antiferromagnetic state is crucial to exploit the properties of antiferromagnets in future spintronic devices. Antiferromagnetic materials have the potential for ultrafast operation [1], with spin dynamics in the terahertz range, high packing density, due to the absence of stray magnetic fields, and an insensitivity to magnetic fields [2,3]. Furthermore, low-power operation is possible in antiferromagnetic insulators (AFM-Is) due to long spin diffusion lengths [4] and the theoretical prediction of superfluid spin transport [5].Recently, the electrical reading of the Néel order (n) orientation in AFM-Is was demonstrated via spin Hall magnetoresistance (SMR) [6-10], a magnetoresistive effect depending on the mutual orientation of the magnetic order and an interfacial spin accumulation μs. However, one of the main challenges faced by AFM spintronics is the reliable electrical writing of the orientation of n. One possible approach exploits staggered Néel spin orbit torques [11], creating an effective field of opposite sign on each magnetic sublattice. However, these torques rely on special material requirements, which has limited their application to the conducting AFMs CuMnAs and Mn2Au [12][13][14][15][16]. Another approach would be to use the non-staggered, antidamping-like torque exerted by a spin accumulation at the interface of a heavy metal and an AFM-I. A charge current in the heavy metal layer can generate a transverse spin current via the spin Hall effect, creating antidamping-like torques in the antiferromagnet.The possibility of such switching was demonstrated in NiO(001)/Pt and Pt/NiO(111)/Pt [17,18], but the mechanisms are still debated. One of the possible mechanisms relies on spin-current induced domain wall (DW) motion [19], predicting that DWs with opposite chirality are driven in opposite directions, thus excluding the electrical signature of the switching when DWs with opposite chirality are equally probable. A second mechanism [18], based on the coherent rotation of n, predicts a current threshold ten times larger than that found experimentally. A third mechanism, based on field-like torques acting on uncompensated interfacial spins, requires perfectly flat interfaces [17]. Currently, none of these provides a consistent explanation of the effect.In this work we realize reliable current-induced switching in epitaxial antiferromagnetic NiO/Pt bilayers. We show that the magnetic state of ...

We report the observation of the three-dimensional angular dependence of the spin Hall magnetoresistance (SMR) in a bilayer of the epitaxial antiferromagnetic insulator NiO(001) and the heavy metal Pt, without any ferromagnetic element. The detected angular-dependent longitudinal and transverse magnetoresistances are measured by rotating the sample in magnetic fields up to 11 T, along three orthogonal planes (xy-, yz-and xz-rotation planes, where the z-axis is orthogonal to the sample plane). The total magnetoresistance has contributions arising from both the SMR and ordinary magnetoresistance. The onset of the SMR signal occurs between 1 and 3 T and no saturation is visible up to 11 T. The three-dimensional angular dependence of the SMR can be explained by a model considering the reversible field-induced redistribution of magnetostrictive antiferromagnetic S-and T-domains in the NiO(001), stemming from the competition between the Zeeman energy and the elastic clamping effect of the non-magnetic MgO substrate. From the observed SMR ratio, we estimate the spin mixing conductance at the NiO/Pt interface to be greater than 2x10 14 Ω -1 m -2 . Our results demonstrate

We demonstrate that we can determine the antiferromagnetic anisotropies and the bulk Dzyaloshinskii-Moriya fields of the insulating iron oxide hematite, α-Fe2O3, using a surface sensitive spin-Hall magnetoresistance (SMR) technique. We develop an analytical model that in combination with SMR measurements, allow for the identification of the material parameters of this prototypical antiferromagnet over a wide range of temperatures and magnetic field values. Using devices with different orientations, we demonstrate that the SMR response strongly depends on the direction of the charge current with respect to the magneto-crystalline anisotropies axis. We show that we can extract the anisotropies over a wide temperature range including across the Morin phase transition. We observe that the electrical response is dominated by the orientation of the antiferromagnetic Néel order parameter, rather than by the emergent weak magnetic moment. Our results highlight that the surface sensitivity of the SMR allows accessing the magnetic anisotropies of antiferromagnetic crystals and in particular thin films where other methods to determine anisotropies such as bulk-sensitive magnetic susceptibility measurements do not provide sufficient sensitivity.Antiferromagnets possess a number of intriguing and promising properties for electronic devices, which include a vanishing net moment and thus insensitivity to large magnetic fields [1] and a characteristic terahertz frequency dynamics [2]. However, antiferromagnets are challenging to probe. Since the pioneering work of Louis Néel [1], they have remained the subject of fundamental studies that have mainly relied on synchrotron based facilities for measurements [3]. In recent years, various new effects were discovered which enable more easy and efficient ways to probe and manipulate the antiferromagnetic (or Néel) vector by electrical current [4][5][6]. The Néel vector can be manipulated by electrical fields in magnetoelectric materials like Cr2O3 [7] or multiferroics like BiFeO3 [8], by bulk spin-galvanic effects in conducting antiferromagnets [9,10], or by interfacial spin-orbit torques in multilayers with the insulating NiO [11][12][13]. For magneto-transport measurements, effects that are even functions of the magnetic order parameter like anisotropic [14,15] and spin-Hall magnetoresistance (SMR) [16][17][18] could probe the antiferromagnetic state and detect switching events [11][12][13]. However, it is not obvious how one can extract the equilibrium state of an antiferromagnet and in particular determine from the field dependence of the SMR key magnetic properties such as the anisotropy values that are otherwise difficult to ascertain.The SMR technique can probe the magnetic state of bilayer systems consisting of a ferromagnetic or an antiferromagnetic insulator and a heavy metal. In the simple models [15,22,28], the longitudinal SMR signal ΔR is proportional to (1 − ( · µ) 2 ) for a ferromagnet, and (1 − ( · µ) 2 ) for an antiferromagnet (where the unit vector μ of spin-accumula...