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We present a detailed analysis on mode evolution of grating-coupled surface plasmonic polaritons (SPPs) on a conical metal tip based on the guided-wave theory. The eigenvalue equations for SPPs modes are discussed, revealing that cylindrical metal waveguides only support TM 01 and HE m1 surface modes. During propagation on the metal tip, the grating-coupled SPPs are converted to HE 31 , HE 21 , HE 11 and TM 01 successively, and these modes are sequentially cut off except TM 01 . The TM 01 mode further propagates with drastically increasing effective mode index and is converted to localized surface plasmons (LSPs) at the tip apex, which is responsible for plasmonic nanofocusing. The gap-mode plasmons can be excited with the focusing TM 01 mode by approaching a metal substrate to the tip apex, resulting in further enhanced electric field and reduced size of the plasmonic focus.

We theoretically study a particular plasmonic structure with stereo nanoholes array in metallic film, which has remarkable abilities to manipulate the optical polarizations at optical frequencies. The main property is that any linear polarization states including a complete 90° optical rotation can be obtained in transmission by proper structural design in combination of enhanced transmission efficiency. Together with the polarization change, surface plasmon propagation bounded on the surface of transmission side also can be modulated. Furthermore, an analytical Coupled Mode Method (CMM) is developed by introducing a frequency dependent coupling coefficient to describe such optical rotation property in stereo plasmonic systems.

Tip-based plasmonic nanofocusing, which delivers light into a nanoscale region and achieves localized electromagnetic (EM) field enhancement beyond the diffraction limit, is highly desired for light-matter interaction-based super-resolution imaging. Here, we present the plasmonic nanofocusing at the apex of a silver (Ag)-coated fiber tip with the internal illumination of a radial vector mode (RVM) generated directly in an optical fiber based on an acoustically-induced fiber grating (AIFG). As illustrated by theoretical calculation, a picture of the nanofocusing plasmonic tip given by analyzing the mode conversion process that the surface plasmon polariton (SPP) mode excited via the radial polarization optical mode can propagate to the apex of the plasmonic tip for nanofocusing because it is not cut off as the tip radius decreases; while the SPP mode which transited from the linear polarization optical mode cannot propagate to the tip apex for nanofocusing because it is cut off as the tip radius decreases. The electric field intensity enhancement factor $|{\rm{E}}_{{\rm{apex}}}^{\rm{2}}|/|{\rm{E}}_{{\rm{input}}}^{\rm{2}}|$ of a plasmonic tip with a tip radius of 20 nm was calculated to be ~2 × 103. Furthermore, the electric field enhancement characteristic at the tip apex was also experimentally verified by using surface-enhanced Raman spectroscopy (SERS). The Raman scattering intensity was observed to be ~15 times as strong as that with internal illumination using the linear polarization mode (LPM), revealing their significantly different nanofocusing characteristics. A Raman sensitivity of 10−14m was achieved for the target analyte of malachite green (MG), denoting significant electric field enhancement and effective plasmonic nanofocusing. The energy conversion efficiency of the radial polarization optical mode to the corresponding SPP mode at the tip apex was measured to be ~17%. This light delivery technique can be potentially further exploited in near-field microscopy with improved resolution and conversion efficiency.

A plasmon-induced hot-electron photodetector based on silicon nanopillar array is developed. The nanostructure is fabricated by reactive ion etching with a monolayer of self-assembled polystyrene nanosphere in hexagonal close-packed lattice as the mask. Light absorption and hotelectron generation are mainly enhanced by the surface plasmon polaritons formed at the surface of the gold film on the nanopillar sidewalls. The photoresponse spans two telecom wavebands, viz. the range of 1250-1600 nm, and has a value of 2.5 mA W −1 at 1310 nm. The proposed silicon nanopillar-based hot-electron infrared detector has great potentials for device integration in silicon photonics relying on the economic large-area fabrication process.

Optical chirality enhancement is highly demanded for enantioselective interaction of circularly polarized light with chiral molecules. The chirality enhancement in the coaxial air hole of a hollow silicon disk depends on three aspects, namely, the enhancements of electric and magnetic fields and a factor determined by the phases of their field components. In the spectral regime of dipole resonances, maximum chirality enhancement with sign consistency and uniform spatial distribution in the air hole can be obtained in association with both magnetic dipole resonance and anapole. Due to dipolar interference, the chirality is nulled at their coincidence, around which the sign of chirality is reversed. Maximum chirality with both positive and negative signs can be found between magnetic dipole resonance and anapole in the vicinity of their coincidence. This situation is maintained under size scaling so that the operation wavelength can be broadly tuned. The optical chirality can be further improved by merely adjusting the hole radius, by which the optimal spatially averaged optical chirality enhancement factor can reach 39 and −23. The simple strategy for optimizing Mie resonators presented in this work may benefit the design of Mie resonator‐based achiral metasurfaces for chirality detection application.

Au-nanoparticle (Au-NP) substrates for surface-enhanced Raman spectroscopy (SERS) were fabricated by grid-like scanning a Au-film using a femtosecond pulse. The Au-NPs were directly deposited on the Au-film surface due to the scanning process. The experimentally obtained Au-NPs presented local surface plasmon resonance effect in the visible spectral range, as verified by finite difference time domain simulations and measured reflection spectrum. The SERS experiment using the Au-NP substrates exhibited high activity and excellent substrate reproducibility and stability, and a clearly present Raman spectra of target analytes, e.g. Rhodamine-6G, Rhodamine-B and Malachite green, with concentrations down to 10 M. This work presents an effective approach to producing Au-NP SERS substrates with advantages in activity, reproducibility and stability, which could be used in a wide variety of practical applications for trace amount detection.

The interplay of Mie's multipole resonances provides a huge opportunity for discovering new phenomena in nanophotonics and developing nanophotonic devices of new functionalities. One of the keys to this task is to control the spectral overlap or separation between resonances, for which Ag/Si core−shell nanostructures, that is, nanospheres and nanodisks, are proposed here. The Ag core and the dielectric shell have different roles in dominating spherical electric dipole (ED) and electric quadrupole (EQ) resonances with different variational trends to the change of the structural parameter such as the core radius. Thus, the EQ and ED may be decoupled in a great spectral separation, such that an excellent anapole can be achieved and lies in a broad valley of the scattering spectrum. The anapole mode displays a perfect far-field radiation pattern of the Cartesian ED and toroidal dipole with destructive interference and radiates more than 70 times less than that of the solid nanodisk of the same size. Only one tightly focused radially polarized beam is needed for illumination in order to avoid excitation of magnetic-type resonances. This work of the spectral characteristics of Ag/Si core−shell nanoparticles provides detailed physical insight into experimental demonstration of nonradiating scatterers and suggests a scheme to study the particular electromagnetic modes in a hybrid nanostructure.