Planar optics constructed from subwavelength artificial atoms have been suggested as a route to the physical realization of steganography with controlled intrinsic redundancy at single-pixel levels. Unfortunately, two-dimensional geometries with uniform flat profiles offer limited structural redundancy and make it difficult to create advanced crypto-information in multiplexed physical divisions. Here, we reveal that splashing three-dimensional (3D) plasmonic nanovolcanoes could allow for a steganographic strategy in angular anisotropy, with high resolution, full coloration, and transient control of structural profiles. Highly reproducible 3D morphologies of volcanic nanosplashes are demonstrated by creating a standardized recipe of laser parameters. Such single nanovolcanoes can be well controlled individually at different splashing stages and thus provide a lithography-free fashion to access various spectral responses of angularly coordinated transverse and vertical modes, leading to the full-range coloration. This chip-scale demonstration of steganographic color images in angular anisotropy unfolds a long-ignored scheme for structured metasurfaces and thereby provides a paradigm for information security and anticounterfeiting.

A new level of anisotropic plasmonic laser printing for aluminum multifunctional metasurfaces.

In this letter, a detecting method for the magneto-optical constant is presented by using weak measurements. The photonic spin Hall effect (PSHE), which manifests itself as spin-dependent splitting, is introduced to characterize the magneto-optical constant, and a propagation model to describe the quantitative relation between the magneto-optical constant and the PSHE is established. According to the amplified shift of the PSHE detected by weak measurements, we determinate the magneto-optical constant of the Fe film sample. The Kerr rotation is measured via the standard polarimetry method to verify the rationality and feasibility of our method. These findings may provide possible applications in magnetic physics research.

The emerging monolayer transition metal dichalcogenides have provided an unprecedented material platform for miniaturized opto-electronic devices with integrated functionalities. Although excitonic light–matter interactions associated with their direct bandgaps have received tremendous research efforts, wavefront engineering is less appreciated due to the suppressed phase accumulation effects resulting from the vanishingly small thicknesses. By introducing loss-assisted singular phase behaviour near the critical coupling point, we demonstrate that integration of monolayer MoS2 on a planar ZnO/Si substrate, approaching the physical thickness limit of the material, enables a π phase jump. Moreover, highly dispersive extinctions of MoS2 further empowers broadband phase regulation and enables binary phase-modulated supercritical lenses manifesting constant sub-diffraction-limited focal spots of 0.7 Airy units (AU) from the blue to yellow wavelength range. Our demonstrations downscaling optical elements to atomic thicknesses open new routes for ultra-compact opto-electronic systems harnessing two-dimensional semiconductor platforms with integrated functionalities.

Owing to its good air stability and high refractive index, two-dimensional (2D) noble metal dichalcogenide shows intriguing potential for versatile flat optics applications. However, light field manipulation at the atomic scale is conventionally considered unattainable because the small thickness and intrinsic losses of 2D materials completely suppress both resonances and phase accumulation effects. Here, we demonstrate that losses of structured atomically thick PtSe2 films integrated on top of a uniform substrate can be utilized to create the spots of critical coupling, enabling singular phase behaviors with a remarkable π phase jump. This finding enables the experimental demonstration of atomically thick binary meta-optics that allows an angle-robust and high unit thickness diffraction efficiency of 0.96%/nm in visible frequencies (given its thickness of merely 4.3 nm). Our results unlock the potential of a new class of 2D flat optics for light field manipulation at an atomic thickness.

No abstract

The feasibility of a localized surface plasmon resonance (LSPR) enhanced sensor based on raspberry-like nanosphere functionalized silica microfibers has been proposed and experimentally demonstrated. The extinction of single Ag (or Au) nanoparticles usually occurs at visible wavelengths. Nevertheless, a LSPR enhancement at near infrared wavelengths has been achieved by constructing raspberry-like meso-SiO nanospheres with noble metal nanoparticle cluster coating. The nanosphere coating captures γ-amino-butyric acid (GABA) targets through size selectivity and enhances the sensitivity by the LSPR effect. The gathering of GABA on the sensor surface translates the concentration signal to the information of refractive index (RI). Silica microfiber perceives the RI change and translates it to optical signal. The LSPR effect enhances the optical sensitivity by enhancing the evanescent field on the microfiber surface. This combination presents the lowest limit of detection (LOD) of 10 M (three orders lower than that without LSPR enhancement). It could fully afford the detection of ultra-low GABA concentration fluctuation (which is important for determining a variety of neurological and psychiatric disorders). The inherent advantages of the proposed sensors, including their ultra-sensitivity, low cost, light weight, small size and remote operation ability, provide the potential to fully incorporate them into various biomedical applications.

The ORCID identification number(s) for the author(s) of this article can be found under https://doi.org/10.1002/adom.201900610. Upconversion NanoparticlesOptical multiplexing and encoding based on light-matter interactions in physical dimensions such as polarization, [1][2][3] wavelength, [4][5][6] angular dispersion, [7][8][9] and orbital angular momentum [10][11][12] have been well heralded as an enabling platform for high-security encryption applications in banknotes, ID cards, and so on. [13,14] Among these well-developed optical