Pulsed electrical discharges in a gas–liquid mixture deposit energy into both phases. Here, we propose a model to simulate breakdown in multiphase based on experimental data. Furthermore, we estimated breakdown voltage in each phase and then estimated energy deposition in each phase. Discharge in pure liquid showed a highly stochastic nature, having a wide breakdown voltage distribution, while the mean value closely follows a one term power law as a function of gap spacing. When there is external gas injection to the gap, breakdown voltage increased significantly due to charge dissipation on bubble surface. This effect was simulated to predict breakdown voltage in liquid with gas injection at different rates. A multiphase system model was developed to simulate breakdown in the gas–liquid phase. The model is a superposition of power law and Meek criteria physical models for the liquid and gas phases, respectively, with empirically derived coefficients. Energy deposition into each phase was estimated by this model. The gap spacing is the primary factor determining breakdown voltage and energy distribution. In studied conditions, we were able to predict the breakdown voltage and estimate energy deposition into different phases. When the gap and flow rate vary between 2 and 10 mm and flow rate 0–1 LPM, 50%–93% of electrical energy is deposited into the liquid. This model allows for predicting breakdown voltage in a multiphase. Furthermore, it allows for control of the energy distribution among the phases in a multiphase pulsed discharge system.
This paper reports a plasma reactive oxygen species (ROS) method for decontamination of PPE (N95 respirators and gowns) using a surface DBD source to meet the increased need of PPE due to the COVID-19 pandemic. A system is presented consisting of a mobile trailer (35 m3) along with several Dielectric barrier discharge sources installed for generating a plasma ROS level to achieve viral decontamination. The plasma ROS treated respirators were evaluated at the CDC NPPTL, and additional PPE specimens and material functionality testing were performed at Texas A&M. The effects of decontamination on the performance of respirators were tested using a modified version of the NIOSH Standard Test Procedure TEB-APR-STP-0059 to determine particulate filtration efficiency. The treated Prestige Ameritech and BYD brand N95 respirators show filtration efficiencies greater than 95% and maintain their integrity. The overall mechanical and functionality tests for plasma ROS treated PPE show no significant variations.
Electrical discharges in liquids with and without gas injection was experimentally studied with two circuits (RC and single spark gap). Electrical breakdown could be initiated from the following mechanisms: electrode initiation; impurity initiation; and Taylor cone driven initiation. Discharges initiated by electrodes were observed only with the single spark gap circuit. Impurities and Taylor cones can initiate discharges when using the RC circuit. With the single spark gap circuit, bubbles were nearly stationary in the gap before and during discharges because of the limited time to respond to the electric field growth (dV/dt = 1 kV ns −1 ). Bubbles and impurities gain significant energy and undergo significant dynamic changes with the RC circuit under a long rising time. Charge relaxation time on bubbles or impurities in the fluids were close to 100 ms, which is comparable with the circuit rising time. Bubble dynamics observed include reduced bubble size, increased bubble speed and shape change. Taylor cones were observed on bubble surface using a high-speed camera during multiple discharge events, and usually led to breakdown. Taylor cones develop on a bubble surface through multiple states over a period of 10-500 μs. State one was typically seen on a bubble surface with a sharp tip caused by the residual charge. A single streamer was initiated on the tip of the cone at state two. State three developed multiple bush-like streamers on the cone and usually triggered a breakdown in the gap. Discharge behaviors in liquids were also investigated with the RC circuit at different pulsing frequencies. At a low pulsing frequency (1 Hz), discharge events are independent from each other. When pulsed above 10 Hz, bubbles created in the gap accumulate and participate in the next discharge event. Bubble accumulation results in a cloud where local secondary discharges are observed with a much higher frequency up to a few kHz for several milliseconds.
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