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An electrooxidative direct difunctionalization of internal alkynes with sulfonyl hydrazides has been developed for the construction of sulfonated enethers. In this transformation, metal catalysts and stoichiometric amount of oxidants are...

Linear microphone arrays combined with the minimum variance distortionless response (MVDR) beamformer have been widely studied in various applications to acquire desired signals and reduce the unwanted noise. Most of the existing array systems assume that the desired sources are in the broadside direction. In this paper, we study and analyze the performance of the MVDR beamformer as a function of the source incidence angle. Using the signal-to-noise ratio (SNR) and beampattern as the criteria, we investigate its performance in four different scenarios: spatially white noise, diffuse noise, diffuse-plus-white noise, and point-source-plus-white noise. The results demonstrate that the optimal performance of the MVDR beamformer occurs when the source is in the endfire directions for diffuse noise and point-source noise while its SNR gain does not depend on the signal incidence angle in spatially white noise. This indicates that most current systems may not fully exploit the potential of the MVDR beamformer. This analysis does not only help us better understand this algorithm, but also helps us design better array systems for practical applications.Index Terms-Beamforming, diffuse noise, microphone arrays, minimum variance distortionless response (MVDR) beamformer, noise reduction, spatially white noise, speech enhancement.

High-throughput sequencing and GC-MS (gas chromatography-mass spectrometry) were jointly used to reveal the bacterial succession and metabolite changes during flax (Linum usitatissimum L.) retting. The inoculation of Bacillus cereus HDYM-02 decreased bacterial richness and diversity. This inoculum led to the replacement of Enterobacteriaceae by Bacillaceae. The level of aerobic Pseudomonadaceae (mainly Azotobacter) and anaerobic Clostridiaceae_1 gradually increased and decreased, respectively. Following the addition of B. cereus HDYM-02, the dominant groups were all degumming enzyme producers or have been proven to be involved in microbial retting throughout the entire retting period. These results could be verified by the metabolite changes, either degumming enzymes or their catalytic products galacturonic acid and reducing sugars. The GC-MS data showed a clear separation between flax retting with and without B. cereus HDYM-02, particularly within the first 72 h. These findings reveal the important bacterial groups that are involved in fiber retting and will facilitate improvements in the retting process.

The scalable reduction of sulfoxides to sulfides in a sustainable way remains an unmet challenge. This report discloses an electrochemical reduction of sulfoxides on a large scale (> 10 g)...

Differential microphone array (DMA), a particular kind of sensor array that is responsive to the differential sound pressure field, has a broad range of applications in sound recording, noise reduction, signal separation, dereverberation, etc. Traditionally, an Nth-order DMA is formed by combining, in a linear manner, the outputs of a number of DMAs up to (including) the order of N - 1. This method, though simple and easy to implement, suffers from a number of drawbacks and practical limitations. This paper presents an approach to the design of linear DMAs. The proposed technique first transforms the microphone array signals into the short-time Fourier transform (STFT) domain and then converts the DMA beamforming design to simple linear systems to solve. It is shown that this approach is much more flexible as compared to the traditional methods in the design of different directivity patterns. Methods are also presented to deal with the white noise amplification problem that is considered to be the biggest hurdle for DMAs, particularly higher-order implementations.