We report a silicon photonic refractometric CO(2) gas sensor operating at room temperature and capable of detecting CO(2) gas at atmospheric concentrations. The sensor uses a novel functional material layer based on a guanidine polymer derivative, which is shown to exhibit reversible refractive index change upon absorption and release of CO(2) gas molecules, and does not require the presence of humidity to operate. By functionalizing a silicon microring resonator with a thin layer of the polymer, we could detect CO(2) gas concentrations in the 0-500ppm range with a sensitivity of 6 × 10(-9) RIU/ppm and a detection limit of 20ppm. The microring transducer provides a potential integrated solution in the development of low-cost and compact CO(2) sensors that can be deployed as part of a sensor network for accurate environmental monitoring of greenhouse gases.

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We report observation of optical bistability and enhanced thermal nonlinearity in a graphene-silicon waveguide resonator. Photo-induced Joule heating in the graphene layer gives rise to a temperature increase in the silicon waveguide core and a corresponding thermo-optic shift in the resonance of the Fabry-Perot resonator. Measurement of the nonlinear resonance spectra showed a 9-fold increase in the effective thermal nonlinear index due to the graphene layer compared with a bare silicon waveguide.

Harnessing the full complexity of optical fields requires complete control of all degrees-of-freedom within a region of space and time -an open goal for present-day spatial light modulators (SLMs), active metasurfaces, and optical phased arrays. Here, we solve this challenge with a programmable photonic crystal cavity array enabled by four key advances: (i) near-unity vertical coupling to high-finesse microcavities through inverse design, (ii) scalable fabrication by optimized, 300 mm full-wafer processing, (iii) picometer-precision resonance alignment using automated, closed-loop "holographic trimming", and (iv) out-of-plane cavity control via a high-speed µLED array. Combining each, we demonstrate near-complete spatiotemporal control of a 64-resonator, two-dimensional SLM with nanosecond-and femtojoule-order switching. Simultaneously operating wavelength-scale modes near the space-and time-bandwidth limits, this work opens a new regime of programmability at the fundamental limits of multimode optical control.

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