The meridional transport of water vapor into the High Arctic, accompanied by dry enthalpy and clouds, impacts the surface radiative forcing. The evolution of one such moist intrusion over 9–11 February 2010 is presented. The event is analyzed using a unique blend of measurements including a new pan‐Arctic retrieval of column water vapor from the Microwave Humidity Sounders, water vapor profiles from a Raman lidar and a ground‐based microwave radiometer at the Polar Environment Atmospheric Research Laboratory (PEARL), in Eureka (80°N, 86°W), on Ellesmere Island in the Canadian High Arctic. A radiation model reveals the intrusion is associated with a 17 W m−2 average increase in downwelling longwave irradiance. Optically thin clouds, as observed by the lidar, contribute a further 20 W m−2 to the downwelling longwave irradiance at their peak. Intrusion events are shown to be a regular occurrence in the Arctic winter with implications for the understanding of the mechanisms driving Arctic Amplification.

[1] Aerosols from the Sarychev Peak volcano entered the Arctic region less than a week after the strongest SO 2 eruption on June 15 and 16, 2009 and had, by the first week in July, spread out over the entire Arctic region. These predominantly stratospheric aerosols were determined to be sub-micron in size and inferred to be composed of sulphates produced from the condensation of SO 2 gases emitted during the eruption. Average (500 nm) Sarychev-induced stratospheric optical depths (SOD) over the Polar Environmental Atmospheric Research Laboratory (PEARL) at Eureka (Nunavut, Canada) were found to be between 0.03 and 0.05 during the months of July and August, 2009. This estimate, derived from sunphotometry and integrated lidar backscatter profiles was consistent with averages derived from lidar estimates over Ny-Ålesund (Spitsbergen). The Sarychev SOD e-folding time at Eureka, deduced from lidar profiles, was found to be approximately 4 months relative to a regression start date of July 27. These profiles initially revealed the presence of multiple Sarychev plumes between the tropopause and about 17 km altitude. After about two months, the complex vertical plume structures had collapsed into fewer, more homogeneous plumes located near the tropopause. It was found that the noisy character of daytime backscatter returns induced an artifactual minimum in the temporal, pan-Arctic, CALIOP SOD response to Sarychev sulphates. A depolarization ratio discrimination criterion was used to separate the CALIOP stratospheric layer class into a low depolarization subclass which was more representative of Sarychev sulphates. Post-SAT (post Sarychev Arrival Time) retrievals of the fine mode effective radius (r eff,f ) and the logarithmic standard deviation for two Eureka sites and Thule (Greenland) were all close to 0.25 mm and 1.6 respectively. The stratospheric analogue to the columnar r eff,f average was estimated to be r eff,f (+) = 0.29 mm for Eureka data. Stratospheric, Raman lidar retrievals at Ny-Ålesund, yielded a post-SAT average of r eff,f (+) = 0.27 mm. These results are $50% larger than the background stratospheric-aerosol value. They are also about a factor of two larger than modeling values used in recent publications or about a factor of five larger in terms of (per particle) backscatter cross section.

Abstract. We present recent progress on nighttime retrievals of aerosol and cloud optical properties over the PEARL (Polar Environmental Atmospheric Research Laboratory) station at Eureka (Nunavut, Canada) in the High Arctic (80 • N, 86 • W). In the spring of 2011 and 2012, a star photometer was employed to acquire aerosol optical depth (AOD) data, while vertical aerosol and cloud backscatter profiles were measured using the CANDAC Raman Lidar (CRL). We used a simple backscatter coefficient threshold (β thr ) to distinguish aerosols from clouds and, assuming that aerosols were largely fine mode (FM)/sub-micron, to distinguish FM aerosols from coarse mode (CM)/super-micron cloud or crystal particles. Using prescribed lidar ratios, we computed FM and CM AODs that were compared with analogous AODs estimated from spectral star photometry. We found (β thr dependent) coherences between the lidar and star photometer for both FM events and CM cloud and crystal events with averaged, FM absolute differences being <∼ 0.03 when associated R 2 values were between 0.2 and 0.8. A β thr sensitivity study demonstrated that zero crossing absolute differences and R 2 peaks were in comparable regions of the β thr range (or physical reasons were given for their disparity). The utility of spectral vs. temporal cloud screening of star photometer AODs was also illustrated. In general our results are critical to building confidence in the physical fidelity of derived, weak amplitude, star photometry AODs and, in turn, towards the development of AOD climatologies and validation databases for polar winter models and satellite sensors.

Abstract. As a consequence of dynamically variable meteorological conditions, springtime Arctic ozone levels exhibit significant interannual variability in the lower stratosphere. In winter 2011, the polar vortex was strong and cold for an unusually long time. Our research site, located at Eureka, Nunavut, Canada (80.05 • N, 86.42 • W), was mostly inside the vortex from October 2010 until late March 2011. The Bruker 125HR Fourier transform infrared spectrometer installed at the Polar Environment Atmospheric Research Laboratory at Eureka acquired measurements from 23 February to 6 April during the 2011 Canadian Arctic Atmospheric Chemistry Experiment Validation Campaign. These measurements showed unusually low ozone, HCl, and HNO 3 total columns compared to the previous 14 yr. To remove dynamical effects, we normalized these total columns by the HF total column. The normalized values of the ozone, HCl, and HNO 3 total columns were smaller than those from previous years, and confirmed the occurrence of chlorine activation and chemical ozone depletion. To quantify the chemical ozone loss, a three-dimensional chemical transport model, SLIMCAT, and the passive subtraction method were used. The chemical ozone depletion was calculated as the mean percentage difference between the measured ozone and the SLIMCAT passive ozone, and was found to be 35 %.

Abstract. The Canadian Network for the Detection of Atmospheric Change (CANDAC) Rayleigh-Mie-Raman lidar (CRL) at Eureka, Nunavut, has measured tropospheric clouds, aerosols, and water vapour since 2007. In remote and meteorologically significant locations, such as the Canadian High Arctic, the ability to add new measurement capability to an existing well-tested facility is extremely valuable. In 2010, linear depolarization 532 nm measurement hardware was installed in the lidar's receiver. To minimize disruption in the existing lidar channels and to preserve their existing characterization so far as is possible, the depolarization hardware was placed near the end of the receiver cascade. The upstream optics already in place were not optimized for preserving the polarization of received light. Calibrations and Mueller matrix calculations are used to determine and mitigate the contribution of these upstream optics on the depolarization measurements. The results show that with appropriate calibration, indications of cloud particle phase (ice vs. water) through the use of the depolarization parameter are now possible to a precision of ±0.05 absolute uncertainty (≤ 10 % relative uncertainty) within clouds at time and altitude resolutions of 5 min and 37.5 m respectively, with higher precision and higher resolution possible in select cases. The uncertainty is somewhat larger outside of clouds at the same altitude, typically with absolute uncertainty ≤ 0.1. Monitoring changes in Arctic cloud composition, including particle phase, is essential for an improved understanding of the changing climate locally and globally.