We present recent measurements of absolute electron-impact ionization cross sections for Be-like C iii, N iv, and O v forming Li-like C iv, N v, and O vi. The measurements were taken using the crossed-beams apparatus at Oak Ridge National Laboratory. A gas cell beam attenuation method was used to independently measure the metastable fractions present in the ion beams. The measured ionization cross sections were compared with calculations using the R-matrix with pseudostates and distorted-wave theoretical methods. Best agreement is found with the R-matrix with pseudostates cross sections results that account for the metastable fractions inferred from the gas attenuation measurements. We present a set of recommended rate coefficients for electron-impact single ionization from the ground state and metastable term of each ion.
This paper presents results concerning measurements of the dissociative recombination (DR) of dihydrogen sulfide ions. In combination with the ion storage ring CRYRING an imaging technique was used to investigate the breakup dynamics of the three-body channel in the DR of 32SD2(+). The two energetically available product channels S(3P) + 2D(2S) and S(1D) + 2D(2S) were both populated, with a branching fraction of the ground-state channel of 0.6(0.1). Information about the angle between the two deuterium atoms upon dissociation was obtained together with information about how the available kinetic energy was distributed between the two light fragments. The recombination cross sections as functions of energy in the interval of 1 meV to 0.3 eV in the center-of-mass frame are presented for 34SH2(+). The thermal rate coefficient for the DR of 34SH2(+) was determined to be (4.8+/-1.0) x 10(-7)(T/300)(-0.72+/-0.1) cm3 s(-1) over this interval.
The time delay in fission induced by bombardment of W with 180 MeV 32S, 240-255 MeV 48Ti, and 315-375 MeV 58Ni has been measured by observation of crystal blocking. There is a clear narrowing and a small increase in the minimum yield of the angular dips for fission compared with scaled dips for elastically scattered ions. This is interpreted as a fission delay of about 2 as, only weakly dependent on energy and atomic number. The delay is longer by 1 to 2 orders of magnitude than obtained from standard interpretations of measurements of prescission neutrons and giant-dipole-resonance gamma rays and from calculations of the nuclear dynamics in heavy-ion reactions.
Absolute cross sections for electron-impact dissociation of CH ϩ producing C ϩ fragment ions were measured in the 3-100 eV range using a crossed electron-ion beams technique with total uncertainties of about 10% near the cross-section peak. Although the measured energy dependence agrees well with two sets of storage ring measurements, the magnitude of the present results lies about 15-25 % below the other results at the crosssection peak near 40 eV. Below 10 eV, the present data tend to exceed the storage ring data, consistent with the presence of excited states in the CH ϩ ion beam. For energies above 29 eV, the cross sections should also include contributions from dissociative ionization, though no clear onset of this channel is evident in any of the three sets of measured data.
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