Nanocomposite films containing Ag nanoparticles embedded in a polymer matrix of Teflon AF, poly(methyl methacrylate) (PMMA) and Nylon 6 were prepared by vapour phase co-deposition in high vacuum. A large variation of the particle plasmon resonance frequency in the visible region was obtained by increasing the Ag volume fraction from 4-80%. The metal volume fraction was measured by energy dispersive x-ray spectrometry (EDX) and the film thickness was measured by surface profilometry. The position, width and strength of the plasmon resonance depend strongly on the metal filling factor, cluster size and interparticle distance. The microstructure of the nanocomposites (shape, size, size distribution and interparticle separation of metal clusters) was determined by transmission electron microscopy. The effect of the surrounding dielectric medium on the optical properties of nanocomposites was investigated by comparing the Teflon AF/Ag, PMMA/Ag and Nylon/Ag composites.
Thin multilayer films of sputtered polytetrafluoroethylene (Teflon) and Fe54Ni27Co19 with different layer thicknesses were prepared by vapor-phase tandem deposition. The films show ferromagnetic resonance frequencies from 3.0to4.7GHz and a high-frequency permeability in the range from 100 to 175, while having negligible losses up to 700MHz and a quality factor Q up to 12 at 1GHz. Thus these films could be promising candidates as high-frequency components used, for example, in mobile communication electronics.
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