Relaxation of complex resonances studied in our recent work on XUV-NIR pump-probe spectroscopy of N2 and naphthalene is affected by quantum interferences. Here were explore control of the relaxation by shaped NIR pulses.
Time-resolved photoelectron spectropscopy (TRPES) allows tracking ultrafast molecular relaxtion through conical intersections. Here, the implementaion of TRPES for solvated organic molecules is presented and applied to relaxation of aminoazobenzenes as well as several bio-mimetic photoactuators.
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