We report on time-modulated two-body weak decays observed in the orbital electron capture of hydrogenlike 140 Pr 59+ and 142 Pm 60+ ions coasting in an ion storage ring. Using non-destructive single ion, time-resolved Schottky mass spectrometry we found that the expected exponential decay is modulated in time with a modulation period of about 7 seconds for both systems. Tentatively this observation is attributed to the coherent superposition of finite mass eigenstates of the electron neutrinos from the weak decay into a two-body final state.

Nuclear deformation effects on the binding energies in heavy ions are investigated. Approximate formulas for the nuclear-size correction and the isotope shift for deformed nuclei are derived. Combined with direct numerical evaluations, these formulas are employed to reanalyse experimental data on the nuclear-charge-distribution parameters in $^{238}\textrm{U}$ and to revise the nuclear-size corrections to the binding energies in H- and Li-like $^{238}\textrm{U}$. As a result, the theoretical uncertainties for the ground-state Lamb shift in $^{238}\textrm{U}^{91+}$ and for the $2p_{1/2}-2s$ transition energy in $^{238}\textrm{U}^{89+}$ are significantly reduced. The isotope shift of the $2p_{j}-2s$ transition energies for $^{142}\textrm{Nd}^{57+}$ and $^{150}\textrm{Nd}^{57+}$ is also evaluated including nuclear size and nuclear recoil effects within a full QED treatment.Comment: 19 pages, 5 table

Electrons bound in highly charged heavy ions such as hydrogen-like bismuth 209Bi82+ experience electromagnetic fields that are a million times stronger than in light atoms. Measuring the wavelength of light emitted and absorbed by these ions is therefore a sensitive testing ground for quantum electrodynamical (QED) effects and especially the electron–nucleus interaction under such extreme conditions. However, insufficient knowledge of the nuclear structure has prevented a rigorous test of strong-field QED. Here we present a measurement of the so-called specific difference between the hyperfine splittings in hydrogen-like and lithium-like bismuth 209Bi82+,80+ with a precision that is improved by more than an order of magnitude. Even though this quantity is believed to be largely insensitive to nuclear structure and therefore the most decisive test of QED in the strong magnetic field regime, we find a 7-σ discrepancy compared with the theoretical prediction.

Isotope shifts in dielectronic recombination spectra were studied for Li-like A Nd 57+ ions with A=142 and A=150. From the displacement of resonance positions energy shifts δE 142,150 (2s − 2p 1/2 ) = 40.2(3)(6) meV ((stat)(sys)) and δE 142,150 (2s − 2p 3/2 ) = 42.3(12)(20) meV of 2s − 2p j transitions were deduced. An evaluation of these values within a full QED treatment yields a change in the mean-square charge radius of 142,150 δ r 2 = -1.36(1)(3) fm 2 . The approach is conceptually new and combines the advantage of a simple atomic structure with high sensitivity to nuclear size.

Abstract. The rate coefficient for radiative and dielectronic recombination of beryllium-like magnesium ions was measured with high resolution at the Heidelberg heavy-ion storage ring TSR. In the electron-ion collision energy range 0-207 eV resonances due to 2s → 2p (∆N = 0) and 2s → 3l (∆N = 1) core excitations were detected. At low energies below 0.15 eV the recombination rate coefficient is dominated by strong 1s 2 (2s 2p 3 P) 7l resonances with the strongest one occuring at an energy of only 21 meV. These resonances decisively influence the Mg  recombination rate coefficient in a low temperature plasma. The experimentally derived Mg  dielectronic recombination rate coefficient (±15% systematical uncertainty) is compared with the recommendation by Mazzotta et al. (1998, A&AS, 133, 403) and the recent calculations by Gu (2003, ApJ, 590, 1131 and by Colgan et al. (2003, A&A, 412, 597). These results deviate from the experimental rate coefficient by 130%, 82% and 25%, respectively, at the temperature where the fractional abundance of Mg  is expected to peak in a photoionized plasma. At this temperature a theoretical uncertainty in the 1s 2 (2s 2p 3 P) 7l resonance positions of only 100 meV would translate into an uncertainty of the plasma rate coefficient of almost a factor 3. This finding emphasizes that an accurate theoretical calculation of the Mg  recombination rate coefficient from first principles is challenging.

Term energies for dielectronic-recombination Rydberg resonances below 0.07 eV are determined for Sc18+ with absolute accuracies below 0.0002 eV by electron collision spectroscopy in an ion storage ring, using the twin-electron-beam technique and a cryogenic photocathode. The lithiumlike 2s_{1/2}-2p_{3/2} transition energy for Z=21 is determined to 4.6 ppm, less than 1% of the few-body effects on radiative corrections. Features from the hyperfine structure of the 2s state could be resolved in the dielectronic-recombination spectrum.

We propose to install a storage ring at an ISOL-type radioactive beam facility for the first time. Specifically, we intend to install the heavy-ion, low-energy ring TSR at the HIE-ISOLDE facility in CERN, Geneva. Such a facility will provide a capability for experiments with stored secondary beams that is unique in the world. The envisaged physics programme is rich and varied, spanning from investigations of nuclear groundstate properties and reaction studies of astrophysical relevance, to investigations with highly-charged ions and pure isomeric beams. The TSR can also be used to remove isobaric contaminants from stored ion beams and for systematic studies within the neutrino beam programme. In addition to experiments performed using beams recirculating within the ring, cooled beams can also be extracted and exploited by external spectrometers for high-precision measurements. The existing TSR, which is presently in operation at the Max-Planck Institute for Nuclear Physics in Heidelberg, is well-suited and can be employed for this purpose. The physics cases, technical details of the existing ring facility and of the beam requirements at HIE-ISOLDE, together with the cost, time and manpower estimates for the transfer, installation and commissioning of the TSR at ISOLDE are discussed in the present technical design report.

Recent spectroscopic models of active galactic nuclei (AGN) have indicated that the recommended electronion recombination rate coefficients for iron ions with partially filled M-shells are incorrect in the temperature range where these ions form in photoionized plasmas. We have investigated this experimentally for Fe XIV forming Fe XIII. The recombination rate coefficient was measured employing the electron-ion merged beams method at the Heidelberg heavy-ion storage-ring TSR. The measured energy range of 0 − 260 eV encompassed all dielectronic recombination (DR) 1s 2 2s 2 2p 6 3l 3l ′ 3l ′′ nl ′′′ resonances associated with the 3p 1/2 → 3p 3/2 , 3s → 3p, 3p → 3d and 3s → 3d core excitations within the M-shell of the Fe XIV (1s 2 2s 2 2p 6 3s 2 3p) parent ion. This range also includes the 1s 2 2s 2 2p 6 3l 3l ′ 4l ′′ nl ′′′ resonances associated with 3s → 4l ′′ and 3p → 4l ′′ core excitations. We find that in the temperature range 2-14 eV, where Fe XIV is expected to form in a photoionized plasma, the Fe XIV recombination rate coefficient is orders of magnitude larger than previously calculated values.