This work introduces multi-material liquid printing as an enabling technology for designing programmed shape-shifting silicones. The goal of this research is to provide a readily available, scalable and customized approach at producing responsive 4D printed structures for a wide range of applications. Hence, the methodology allows customization at each step of the procedure by intervening either on the material composition and/or on the design and fabrication strategies for the production of responsive components. A significant endeavour is initiated to develop and engineer two different material systems that enable shape-shifting: silicone-ethanol composites and polyvinyl siloxane swelling rubbers. The printed samples successfully comply with the expected swelling behaviour through a variety of printed test patterns.
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