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The Australian bushfires around the turn of the year 2020 generated an unprecedented perturbation of stratospheric composition, dynamical circulation and radiative balance. Here we show from satellite observations that the resulting planetary-scale blocking of solar radiation by the smoke is larger than any previously documented wildfires and of the same order as the radiative forcing produced by moderate volcanic eruptions. A striking effect of the solar heating of an intense smoke patch was the generation of a self-maintained anticyclonic vortex measuring 1000 km in diameter and featuring its own ozone hole. The highly stable vortex persisted in the stratosphere for over 13 weeks, travelled 66,000 km and lifted a confined bubble of smoke and moisture to 35 km altitude. Its evolution was tracked by several satellite-based sensors and was successfully resolved by the European Centre for Medium-Range Weather Forecasts operational system, primarily based on satellite data. Because wildfires are expected to increase in frequency and strength in a changing climate, we suggest that extraordinary events of this type may contribute significantly to the global stratospheric composition in the coming decades.

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Most chemistry-climate models show an intensification of the Brewer-Dobson circulation (BDC) in the stratosphere associated with increasing greenhouse gas emissions and ozone depletion in the last decades, but this trend remains to be confirmed in observational data. In this work the evolution of the advective BDC for the period 1979-2012 is evaluated and compared in three modern reanalyses (ERA-Interim, MERRA, and JRA-55). Three different estimates of the BDC are computed for each reanalysis, one based on the definition of the residual circulation and two indirect estimates derived from momentum and thermodynamic balances. The comparison among the nine estimates shows substantial uncertainty in the mean magnitude (∼40%) but significant common variability. The tropical upwelling series show variability linked to the stratospheric quasi-biennial oscillation and to El Niño-Southern Oscillation (ENSO) and also reflect extreme events such as major sudden stratospheric warmings and volcanic eruptions. The trend analysis suggests a strengthening of tropical upwelling of around 2-5%/decade throughout the layer 100-10 hPa. The global spatial structure of the BDC trends provides evidence of an overall acceleration of the circulation in both hemispheres, with qualitative agreement among the estimates. The global BDC trends are mainly linked to changes in the boreal winter season and can be tracked to long-term increases in the resolved wave drag in both hemispheres.

Wave‐induced Lagrangian fluctuations of temperature and vertical velocity in the lower stratosphere are quantified using measurements from superpressure balloons (SPBs). Observations recorded every minute along SPB flights allow the whole gravity wave spectrum to be described and provide unprecedented information on both the intrinsic frequency spectrum and the probability distribution function of wave fluctuations. The data set has been collected during two campaigns coordinated by the French Space Agency in 2010, involving 19 balloons over Antarctica and 3 in the deep tropics. In both regions, the vertical velocity distributions depart significantly from a Gaussian behavior. Knowledge on such wave fluctuations is essential for modeling microphysical processes along Lagrangian trajectories. We propose a new simple parameterization that reproduces both the non‐Gaussian distribution of vertical velocities (or heating/cooling rates) and their observed intrinsic frequency spectrum.

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The Brewer-Dobson mean circulation and its variability are investigated in the ERA-Interim over the period 1989-2010 by using an off-line Lagrangian transport model driven by analysed winds and heating rates. <br><br> At low and mid-latitudes, the mean age of air in the lower stratosphere is in good agreement with ages derived from aircraft, high altitude balloon and satellite observations of long-lived tracers. At high latitude and in the upper stratosphere, we find, however that the ERA-Interim ages exhibit an old bias, typically of one to two years. <br><br> The age spectrum exhibits a long tail except in the low tropical stratosphere which is modulated by the annual cycle of the tropical upwelling. The distribution of ages and its variability is consistent with the existence of two separate branches, shallow and deep, of the Brewer-Dobson circulation. Both branches are modulated by the tropical upwelling and the shallow branch is also modulated by the subtropical barrier. <br><br> The variability of the mean age is analysed through a decomposition in terms of annual cycle, QBO, ENSO and trend. The annual modulation is the dominating signal in the lower stratosphere and is maximum at latitudes greater than 50° in both hemispheres with oldest ages at the end of the winter. The phase of the annual modulation is also reversed between below and above 25 km. The maximum amplitude of the QBO modulation is of about 0.5 yr and is mostly concentrated within the tropics between 25 and 35 km. It lags the QBO wind at 30 unit{hPa} by about 8 months. The ENSO signal is small and limited to the lower northen stratosphere. <br><br> The age trend over the 1989–2010 period, according to this ERA-Interim dataset, is significant and negative, of the order of −0.3 to −0.5 yr dec⁻¹, within the lower stratosphere in the Southern Hemisphere and south of 40° N in the Northern Hemisphere below 25 km. The age trend is positive (of the order of 0.3 yr dec⁻¹) in the mid stratosphere but there is no region of consistent significance. This suggests that the shallow and deep Brewer-Dobson circulations may evolve in opposite directions. <br><br> Finally, we find that the long lasting influence of the Pinatubo eruption can be seen on the age of air from June 1991 until the end of 1993 and can bias the statistics encompassing this period

It is an outstanding issue to what degree trends in stratospheric mean age of air reflect changes in the (slow) residual circulation and how they are affected by (fast) eddy mixing. We present a method to quantify the effects of mixing and residual circulation on mean age trends, based on simulations with the Chemical Lagrangian Model of the Stratosphere (CLaMS) driven by ERA‐Interim reanalysis and on the integrated tracer continuity equation. During 1990–2013, mean age decreases throughout most of the stratosphere, qualitatively consistent with results based on climate model simulations. During 2002–2012, age changes show a clear hemispheric asymmetry in agreement with satellite observations. We find that changes in the residual circulation transit time cannot explain the mean age trends, and including the integrated effect of mixing is crucial. Above about 550 K (about 22 km), trends in the mixing effect on mean age appear to be coupled to residual circulation changes.