Polyvinylcarbazole polymer scintillators with high loading of a bismuth organometallic exhibit good light yields, and are found to be capable of gamma-ray spectroscopy. When activated by a standard fluor, diphenylanthracene, a bismuth-loaded polymer produces ∼12000 photons/MeV, exhibits an emission maximum at 420 nm, a ∼15 ns decay, and energy resolution of 9% at 662 keV is measured. The same bismuth-loaded polymer doped with an iridium complex fluor has an emission maximum of 500 nm, a decay time of 1.2 µs, a light yield of ∼30000 photons/MeV, and energy resolution better than 7% FWHM at 662 keV.
Transparent ceramics combine the scintillation performance of single crystals with the ruggedness and processability of glass. We have developed a versatile, scaleable fabrication method, wherein nanoparticle feedstock is consolidated at temperatures well below melting to form inch-scale phase-pure transparent ceramics with optical scatter of α <0.1 cm -1 . We have fabricated Cerium-doped Gadolinium Garnets with light yields of ~50,000 Ph/MeV and energy resolution of <5% at 662 keV. We have also developed methods to form sheets of the high-Z ceramic scintillator, Europium-doped Lutetium Oxide Bixbyite, producing ~75,000 Ph/MeV for radiographic imaging applications.
Abstract-We are developing new scintillator materials that offer potential for high resolution gamma ray spectroscopy at low cost. Single crystal SrI 2 (Eu) offers ~3% resolution at 662 keV, in sizes of ~1 in 3 . We have developed ceramics processing technology allowing us to achieve cubic inch scale transparent ceramic scintillators offering gamma spectroscopy performance superior to NaI(Tl).We fabricated a bismuth-loaded plastic scintillator that demonstrates energy resolution of ~8% at 662 keV in small sizes.
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