We provide a unified semiclassical approach for thermoelectric responses of any observable represented by an operatorθ that is well-defined in periodic crystals. The Mott relation is established, in the presence of Berry-phase effects, for various physical realizations ofθ in electronic systems, including the familiar case of the electric current as well as the currently controversial cases of the spin polarization and spin current. In our theory the dipole density of a physical quantity emerges and plays a vital role, which contains not only the statistical sum of the dipole moment ofθ but also a Berry-phase correction.
To give a general description of the influences of electric fields or currents on magnetization dynamics, we developed a semiclassical theory for the magnetization implicitly coupled to electronic degrees of freedom. In the absence of electric fields the Bloch electron Hamiltonian changes the Berry curvature, the effective magnetic field, and the damping in the dynamical equation of the magnetization, which we classify into intrinsic and extrinsic effects. Static electric fields modify these as first-order perturbations, using which we were able to give a physically clear interpretation of the current-induced spin-orbit torques. We used a toy model mimicking a ferromagnet-topologicalinsulator interface to illustrate the various effects, and predicted an anisotropic gyromagnetic ratio and the dynamical stability for an in-plane magnetization. Our formalism can also be applied to the slow dynamics of other order parameters in crystalline solids.
We extend the semiclassical Boltzmann formalism for the anomalous Hall effect (AHE) in nondegenerate multiband electron systems to the spin Hall effect (SHE) and unconventional Edelstein effect (UEE, cannot be accounted for by the conventional Boltzmann equation, unlike the conventional Edelstein effect). This extension is confirmed by extending the Kohn-Luttinger density-matrix transport theory in the weak disorder-potential regime. By performing Kubo linear response calculations in a prototypical multiband model, the Boltzmann scaling for the AHE/SHE and UEE is found to be practically valid only if the disorder-broadening of bands is quite smaller than the minimal intrinsic energy-scale around the Fermi level. Discussions on this criterion in various multiband systems are also presented. A qualitative phase diagram is proposed to show the influences of changing independently the impurity density and strength of disorder potential on the AHE/SHE and UEE.
In model studies of the spin/anomalous Hall effect, effective Hamiltonians often serve as the starting point. However, a complete effective quantum theory contains not only the effective Hamiltonian but also the relation linking the physical observables to the canonical ones. In this work we construct the semiclassical Boltzmann transport framework in the weak disorder-potential regime directly in the level of the effective quantum theory, and confirm this construction by formulating a generalized Kohn-Luttinger density matrix transport theory also in this level. The link and difference between the present theory and previous phenomenological Boltzmann, quantum kinetic and usual Kubo-Streda theories are clarified. In the application to a two-dimensional Rashba electron effective model, a nonzero spin Hall effect important in the case of strong Rashba coupling but neglected in previous theories is found.
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