Herein, the role of thermal softening in ultrasonic powder compaction is assessed by comparing the densification behaviors of nominally pure Cu and a thermally stable CuTa alloy. These materials have similar thermal properties, but pure Cu softens at much lower temperatures than does the CuTa alloy. Using a specialized ultrasonic powder compaction setup, in situ measurements of relative density, sonotrode power consumption, and temperature are collected, which together provide a time‐dependent geometric hardening parameter that reflects the structure of the compact. The geometric hardening data for the pure Cu powder reveal three distinct stages of densification: an initial particle rearrangement stage; a jamming transition where strong junctions develop between particles; and a final stage characterized by compatible plastic deformation. By contrast, the geometric hardening data for the thermally stable CuTa powder show that it remains a weak fluidized granular medium, despite experiencing higher normal pressures, oscillation amplitudes, and temperatures. The contrasting behaviors of the Cu and the CuTa powders suggest that a thermally activated jamming transition drives interparticle junction growth and densification in ultrasonic powder compaction.
Ultrasonic additive manufacturing has been used to fabricate laminated composites of commercially pure aluminum and a nanocrystalline nickel–cobalt (nc-NiCo) alloy. The nc-NiCo alloy would not weld to itself but readily welded to aluminum. Thus, by alternating between foils of nc-NiCo and Al, we achieved multi-material laminates with strong interlayer bonding. Electron microscopy showed that the nanoscale grain structure of the nc-NiCo was preserved during deposition and that the nc-NiCo/Al weld interface was decorated with comminuted surface oxides as well as Al–Ni–Co intermetallics. These findings are considered in light of process models of junction growth, interdiffusion, and grain growth, which together reveal how the different pressure- and temperature dependences of these phenomena give rise to a range of processing conditions that maximize bonding while minimizing coarsening and intermetallic formation. This analysis quantitatively demonstrates that using a soft, low melting point interlayer material decouples junction growth at the weld interface from grain growth in the nc-NiCo, expanding the range of optimal processing conditions.
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