After a brief examination of known insulating laser crystals and the stimulated emission channels of their generating activator ions, this article reviews recent advances in the development of novel lasing crystals and ceramics, as well as inorganic and organic nonlinear-laser crystals for χ (3) and cascaded χ (3) ↔ χ (2) frequency converters. Several new modern attractive technologies in the physics and techniques of crystalline lasers are also discussed.Section of the crystal structure of Na3Li (SeO4)

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Spectroscopic, laser, and chi((3)) nonlinear optical properties of tetragonal PbWO(4), NaY(WO(4))(2), CaWO(4), and monoclinic CdWO(4) and ZnWO(4) were investigated. Particular attention was paid to Nd(3+)-doped and undoped PbWO(4) and NaY(WO(4))(2) crystals. Their absorption and luminescence intensity characteristics, including the peak cross sections of induced transitions, were determined. Pulsed and continuous-wave lasing in the two 4F(3/2)-->4I(11/2) and 4F(3/2)-->4I(13/2) channels was excited. For these five tungstates, highly efficient (greater than 50%) multiple Stokes generation and anti-Stokes picosecond generation were achieved. All the observed scattered laser components were identified. These results were analyzed and compared with spectroscopic data from spontaneous Raman scattering. A new crystalline Raman laser based on PbWO(4) was developed for the chi((3)) conversion frequency of 1-microm pump radiation to the first Stokes emission with efficiency up to 40%. We classify all the tungstates as promising media for lasers and neodymium-doped crystals for self-stimulated Raman scattering lasers.

Library of Congress Cataloging-in-Publication Data. Kaminskii, Aleksandr Aleksandrovich. [Lazernye kristally. English] Laser crystals : their physics and properties / Alexander A. Kaminskii. -2nd ed. p. cm. -(Springer series in optical sciences ; v. 14) Translation of: Lazernye kristally. Includes bibliographical references.

We have demonstrated CW one-micron laser oscillation in new ceramic laser material on the base of cubic Nd3+:Y2O3. Slope efficiency of 32% was achieved on an uncoated 1.5 at.% Nd3+:Y2O3 ceramic plate with size of φ14 ×2.7 mm under laser diode end-pumping.

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