We report the fabrication of a photosensor based on as-grown single crystal monolayers of MoS2 synthesized by chemical vapor deposition (CVD). The measurements were performed using Au/Ti leads in a two terminal configuration on CVD-grown MoS2 on a SiO2/Si substrate. The device was operated in air at room temperature at low bias voltages ranging from −2 V to 2 V and its sensing capabilities were tested for two different excitation wavelengths (514.5 nm and 488 nm). The responsivity reached 1.1 mA W−1 when excited with a 514.5 nm laser at a bias of 1.5 V. This responsivity is one order of magnitude larger than that reported from photo devices fabricated using CVD-grown multilayered WS2. A rectifying-effect was observed for the optically excited current, which was four times larger in the direct polarization bias when compared to the reverse bias photocurrent. Such rectifying behavior can be attributed to the asymmetric electrode placement on the triangular MoS2 monocrystal. It is envisioned that these components could eventually be used as efficient and low cost photosensors based on CVD-grown transition metal dichalcogenide monolayers.
This work shows evidence of conventional liquid and polymer molecules doping macroscopic yarns made up of carbon nanotubes (CNT), an effect that is exploited to monitor polymer flow and thermoset curing during fabrication of a structural composite by vacuum infusion. The sensing mechanism is based on adsorption of liquid/polymer molecules after infiltration into the porous fibers. These molecules act as dopants that produce large changes in longitudinal fiber resistance, closely related to the low density of carriers near the Fermi level of bulk samples of CNT fibers, reminiscent of their low‐dimensional constituents. A 25% decrease in fiber resistance upon exposure to electron–donor radicals formed during epoxy vinyl ester polymerization is shown as an example. At later stages of curing the matrix undergoes shrinkage and applies a compressive stress to the fibers. The resulting sharp increase in electrical resistance provides a mechanism for detection of the matrix gel point. The kinetics of resistance change during polymer ingress are related to established models for macromolecular adsorption, thus also enabling prediction of polymer flow. This is demonstrated for vacuum infusion of a 150 cm2 glass fiber laminate composite, with the CNT fiber yarns giving accurate prediction of macroscopic resin flow according to Darcy's law.
Metamaterials are artificial materials that derive their unusual properties from their periodic architecture. Some metamaterials can deform their internal structure to switch between different properties. However, the precise control of these deformations remains a challenge, as these structures often exhibit non-linear mechanical behavior. We introduce a computational and experimental strategy to explore the folding behavior of a range of 3D prismatic building blocks that exhibit controllable multifunctionality. By applying local actuation patterns, we are able to explore and visualize their complex mechanical behavior. We find a vast and discrete set of mechanically stable configurations, that arise from local minima in their elastic energy. Additionally these building blocks can be assembled into metamaterials that exhibit similar behavior. The mechanical principles on which the multistable behavior is based are scale-independent, making our designs candidates for e.g., reconfigurable acoustic wave guides, microelectronic mechanical systems and energy storage systems.
Microwave optomechanical circuits have been demonstrated in the past years to be extremely powerfool tools for both, exploring fundamental physics of macroscopic mechanical oscillators as well as being promising candidates for novel on-chip quantum limited microwave devices. In most experiments so far, the mechanical oscillator is either used as a passive device element and its displacement is detected using the superconducting cavity or manipulated by intracavity fields. Here, we explore the possibility to directly and parametrically manipulate the mechanical nanobeam resonator of a cavity electromechanical system, which provides additional functionality to the toolbox of microwave optomechanical devices. In addition to using the cavity as an interferometer to detect parametrically modulated mechanical displacement and squeezed thermomechanical motion, we demonstrate that parametric modulation of the nanobeam resonance frequency can realize a phase-sensitive parametric amplifier for intracavity microwave photons. In contrast to many other microwave amplification schemes using electromechanical circuits, the presented technique allows for simultaneous cooling of the mechanical element, which potentially enables this type of optomechanical microwave amplifier to be quantum-limited. INTRODUCTIONSuperconducting microwave circuits have been demonstrated to be extremely powerful tools for the fields of quantum information processing 1-3 , circuit quantum electrodynamics 4-8 , astrophysical detector technologies 9 and microwave optomechanics 10-12 . In the latter, microwave fields in superconducting cavities are parametrically coupled to mechanical elements such as suspended capacitor drumheads or metallized nanobeams, enabling high-precision detection and manipulation of mechanical motion. Milestones achieved in the field include sideband-cooling of mechanical oscillators to the quantum ground state 11 , strong coupling between photons and phonons 13 , the generation of non-Gaussian states of motion [14][15][16] or the entanglement between two mechanial oscillators 17 .Recently, there are increasing efforts taken towards building passive and active quantum limited microwave elements for quantum technologies based on microwave optomechanical circuits, connecting the fields of microwave optomechanics, circuit quantum electrodynamics and quantum information science 18-20 . Among the most important developments into this direction are the demonstration of microwave amplification by blue sideband driving in simple optomechanical circuits 21 , and the realization of directional microwave amplifiers 22 as well as microwave circulators 23,24 in more complex multimode systems 25 .Recent theoretical work 26-28 on optomechanical systems with a parametrically driven mechanical oscillator proposed the use of mechanical parametric driving to enable parametric amplification with enhanced bandwidth and reduced added noise, compared to the case of a optomechanical amplifier using a blue-sideband drive 26 . Furthermore, the authors pre...
Rather than depending on material composition to primarily dictate performance metrics, metamaterials can leverage geometry to achieve specific properties of interest. For example, reconfigurable metamaterials have enabled programmable shape transformations, tunable mechanical properties, and energy absorption. While several methods exist to fabricate such structures, they often place severe restrictions on manufacturing materials, or require significant manual assembly. Moreover, these arrays are typically composed of unit cells that are either macro-scale or micro-scale in dimension. Here, the fabrication gap is bridged, and laminate manufacturing is used to develop a method for designing reconfigurable metamaterials at the millimeter-scale, that is compatible with a wide range of materials, and that requires minimal manual assembly. In addition to showing the versatility of this fabrication method, how the use of laminate manufacturing affects the behavior of these multi-component arrays is also characterized. To this end, a numerical model that captures the deformations exhibited by the structures is developed, and an analytic model that predicts the strain of the structure under compressive stress is built. Overall, this approach can be leveraged to develop millimeter-scale metamaterials for applications that require reconfigurable materials, such as in the design of tunable acoustics, photonic waveguides, and electromagnetic devices.
Phone: þ52 55 5950 4275, Fax: þ 52 55 5950 4284Double-helix microstructures consisting of two parallel strands of hundreds of multi-walled carbon nanotubes (MWCNTs) have been synthesized by chemical vapour deposition of ferrocene/toluene vapours on metal substrates. Growth of coiled carbon nanostructures with site selectivity is achieved by varying the duration of thermochemical pretreatment to deposit a layer of SiO x on the metallic substrate. Production of multibranched structures of MWCNTs converging in SiO x microstructure is also reported.In the abstract figure, panel (a) shows a coloured micrograph of a typical double-helix coiled microstructure of MWCNTs grown on SiO x covered steel substrate. Green and blue show each of the two individual strands of MWCNTs. Panel (b) is an amplification of a SiO x microparticle (white) on the tip of the double-stranded coil (green and blue). The microparticle guides the collective growth of hundreds of MWCNTs to form the coiled structure.
Sub‐millimeter robots—microrobots—that can autonomously perform mechanical work at the microscale would radically change new areas of human activity such as micromanipulation, microfabrication, or healthcare. Sets of identical microrobots that can connect into different, larger structures open the possibility for a “universal” microrobotic unit that fulfills a large variety of functions derived from the structure that multiple units can be assembled into. The capability of individual hydrogel microcrawlers to self‐assemble under confinement into periodically ordered planar structures is demonstrated. Subsequently, these can be bound together using light to form a solid porous sheet. The lateral shape of the sheet is imprinted during the binding process. Furthermore, the sheets bend into 3D structures, where the bending direction can be programmed. The resulting structures actuate anisotropically when exposed to heat or laser illumination and can be designed for various modes of operation, such as manipulation or untethered locomotion. The formation of ordered microstructures from individual mobile robots enables easier transport and remote assembly of these structures at the place of interest without the need for direct intervention.
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