Coherent excitations of intricate assemblies of molecules play an important role in natural photosynthesis. Microcavities are wavelength-dimension artificial structures in which excitations can be made to couple through their mutual interactions with confined photon modes. Results for microcavities containing two spatially separated cyanine dyes are presented here, where simultaneous strong coupling of the excitations of the individual dyes to a single cavity mode leads to new eigenmodes, described as admixtures of all three states. These "hybrid" exciton-photon structures are of potential interest as model systems in which to study energy capture, storage, and transfer among coherently coupled molecular excitations.
We describe experiments on a semiconductor microcavity which provide the first demonstration of motional narrowing in semiconductor inter-subband optical transitions. Significant narrowing occurs because of the small mass of the polaritons in a microcavity. The demonstration is made possible by the control provided in a microcavity of the mixing between photon and exciton states, and hence the dispersion of the polariton.
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