“…In such a case, the apparition of this new phase will depend on the degree of supersaturation and on the time elapsed in this state, implying that this may also not happen even if feasible. Experimentally, condensation has been observed in underexpanded jets [157,267,74,15,284,130,123,65,205,184,92] and the appearance of a solid phase is well documented in the RESS (for Rapid Expansion of Supercritical Solution) process where a supercritical fluid is used as a solvent containing a solute which is seen to precipitate during the expansion. However, there is no overall study concerning the appearance of these new phases, as a function of the initial conditions or depending on the fluid involved in the jet, and so this point is still unclear.…”