“…1 The non-linear, multiphoton process of two-photon absorption (TPA) has been gaining greater interest among a number of multidisciplinary areas, particularly in the rapidly developing fields of multiphoton fluorescence imaging, optical data storage and switching, optical sensor protection, telecommunications, laser dyes, 3-D microfabrication and photodynamic therapy (PDT). [2][3][4][5] The demands of such applications exceed properties and reliabilities delivered by current organic materials, underscoring the need for increasingly sophisticated non-linear optical organic materials. Since the probability of a TPA process is proportional to the square of the incident light intensity, photoexcitation is spatially confined to the focal volume.…”