We experimentally demonstrate spectral broadening and shaping of exponentially-decaying nanosecond pulses via nonlinear mixing with a phase-modulated pump in a periodically-poled lithium niobate (PPLN) waveguide. A strong, 1550 nm pulse is imprinted with a temporal phase and used to upconvert a weak 980 nm pulse to 600 nm while simultaneously broadening the spectrum to that of a Lorentzian pulse up to 10 times shorter. While the current experimental demonstration is for spectral shaping, we also provide a numerical study showing the feasibility of subsequent spectral phase correction to achieve temporal compression and re-shaping of a 1 ns mono-exponentially decaying pulse to a 250 ps Lorentzian, which would constitute a complete spectro-temporal waveform shaping protocol. This method, which uses quantum frequency conversion in PPLN with > 100 : 1 signal-to-noise ratio, is compatible with single photon states of light.
IntroductionHybrid quantum networks that combine different physical systems are one approach to achieving the varied functions needed in photonic quantum information processing systems [1]. Unfortunately, the disparate components of such a quantum network may not share the same spectro-temporal properties, leading to an intrinsic incompatibility that can only be overcome via an "adaptation interface." For example, single photon sources based on single quantum emitters like InAs quantum dots [2], nitrogen vacancy centers in diamond [3], and neutral alkali atoms [4] exhibit desirable features such as on-demand generation with the potential for high single photon purity. To interface the emission wavelengths below 1000 nm with the low-loss telecommunications band, quantum frequency conversion interfaces [5,6] have been proposed and developed, both in bulk and on-chip geometries. However, wavelength incompatibility is not the only challenge that needs to be overcome. While the temporal waveform of such two-level quantum emitters is typically a few nanosecond mono-exponential decay, telecommunications networks are better suited to Gaussian and square pulses that are much shorter in duration. Moreover, the bandwidth of quantum memories that are an integral part of the quantum repeater protocol may be either broader or narrower than the bandwidth of the photons [7]. Spectro-temporal shaping of single photons, while preserving their quantum nature, is thus a vital tool for hybrid quantum networks [8,9].