Tuning electronic structures of uranyl fluorides via increasing equatorial pyridyl number and extending pyridyl conjugation

Lv, Chunmei; Wang, Yongming; Bai, Fu‐Quan; Zhang, Hongxing; Pan, Qing‐Jiang

doi:10.1016/j.comptc.2014.11.008

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Architecture Of Qtpy Coordination Complexes1

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2016

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“…In fact, this behavior has also been seen with Co(II) in its complex with the functionalized qtpy 30 , wherein there is some parallel with the binding of EDTA to lighter first-row transition-metal ions. Heavier metal ions have not been a subject of detailed interest; nonetheless, the electronic structures of the monometallic uranyl complexes [(UO 2 )( 17 )F] + and [(UO 2 )( 17 )] 2+ were recently calculated in silico and compared with those of other pyridine analogues . This interest might well increase as a result of the ongoing boom in domains such as catalysis and renewable energy sources (cf.…”

Section: Architecture Of Qtpy Coordination Complexesmentioning

confidence: 99%

Quaterpyridines as Scaffolds for Functional Metallosupramolecular Materials

et al. 2016

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Quaterpyridine (qtpy) ligands have found significant applications as N-heterocyclic scaffolds in self-assembly processes, in particular the formation of various metallosupramolecular architectures, limited, however, by difficulties in their synthesis. Recent progress in the preparative organic and organometallic chemistry of polypyridines has resulted in the elimination of the most serious drawbacks concerning qtpy synthesis, consequently giving rise to a renewed interest in this class of compounds. Herein, we endeavor to define the essential aspects of quaterpyridine chemistry and provide the reader with a perspective on the ways in which this field has begun to flourish.

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Section: Architecture Of Qtpy Coordination Complexesmentioning

confidence: 99%