“…Among the different chalcogenide crystals, Cr 2+ :CdSe is a promising candidate, as its vibronic emission covers the 2.2-3.6 μm spectral range [5][6][7][8], which overlaps the fundamental vibrational transitions of hydrocarbons, water, and other relevant chemical and biological molecules. After the first laser actions in Cr:CdSe crystal [6,7], subsequent demonstrations proved excellent laser efficiencies and wide wavelength tunability both in continuous wave (CW) [9,10] and in gainswitching regimes, using different pump sources such as Tm-doped crystal lasers, diode lasers, and Tm-fiber lasers [9][10][11][12][13][14][15]. However, attempts to develop Cr 2+ :CdSe lasers with higher output power levels have been hampered by the strong sensitivity of CdSe crystal to thermo-optical effects, such as thermal lensing and mode wavefront distortion.…”