2012
DOI: 10.1063/1.4759252
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Transient photoresponse and incident power dependence of high-efficiency germanium quantum dot photodetectors

Abstract: We report a systematic study of time-resolved and power-dependent photoresponse in high-efficiency germanium quantum dot photodetectors (Ge-QD PDs), with internal quantum efficiencies greater than 100 over a broad wavelength, reverse bias, and incident power range. Turn-on and turn-off response times (τ on and τ off) are shown to depend on series resistance, bias, optical power, and thickness (W QD) of the Ge-QD layer, with measured τ off values down to ∼40 ns. Two different photoconduction regimes are observe… Show more

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Cited by 40 publications
(33 citation statements)
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“…An overshoot of the photocurrent was observed when switching on the incident light. This phenomena were also reported previously in polymer, quantum dots, and perovskite‐based optoelectronic devices, which might be attributed to the fast photoabsorption, unique charge transport and potential trapping, and subsequent electric field redistribution in the perovskite film . To identify the response time of IPD, we introduced incident light of 535 nm with frequency of 305 Hz as light source.…”
Section: Resultssupporting
confidence: 73%
“…An overshoot of the photocurrent was observed when switching on the incident light. This phenomena were also reported previously in polymer, quantum dots, and perovskite‐based optoelectronic devices, which might be attributed to the fast photoabsorption, unique charge transport and potential trapping, and subsequent electric field redistribution in the perovskite film . To identify the response time of IPD, we introduced incident light of 535 nm with frequency of 305 Hz as light source.…”
Section: Resultssupporting
confidence: 73%
“…The pure perovskite photodetector also exhibited transient current overshoots (Figure S16, Supporting Information), ruling out the possibility that PDPP3T was the inducement. This phenomenon has already been reported for photodetectors based on germanium QDs and all‐polymer solar cells, and it could be regulated by illumination power density and applied voltage. In our system, the fast photocurrent overshoot followed by decaying to a steady state might be related to the fast photoabsorption, unique charge transport and potential trapping, and subsequent electric field redistribution in the perovskite film.…”
supporting
confidence: 54%
“…For these reasons, Ge has been a widely‐used material for CMOS‐compatible PD fabrication . Apart from its crystalline form, a variety of Ge nanostructures have been investigated for improved optoelectronic performance including Ge QDs embedded in an oxide matrix for high‐efficiency photodetection . The principal advantages of Ge QDs include reduced phonon scattering, leading to longer carrier relaxation times, as well as confinement in all three spatial dimensions that can reduce the dark current, both contributing to higher SNR.…”
Section: Introductionmentioning
confidence: 99%