2021
DOI: 10.1021/acsanm.1c02759
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Three-Dimensional Graphene-Based Foams with “Greater Electron Transferring Areas” Deriving High Gas Sensitivity

Abstract: Graphene foams are promising three-dimensional (3D) architectures with the combination of the intrinsic nature of graphene and unique cellular structures for various realms. Herein, a facile technique is developed by combining supramolecular assembly with lyophilization to functionalize graphene with donor−π-acceptor (D−π-A) molecules and then massively transform the two-dimensional (2D) plane nanosheets into 3D foams. The as-prepared gas sensors work at room temperature (RT) and reveal comprehensive gas sensi… Show more

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Cited by 9 publications
(5 citation statements)
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“…Three-dimensional nanostructured graphene not only inherits some unique properties of two-dimensional graphene but also offers numerous novel features, such as a boosted surface area, rapid gas diffusion, and abundant reaction sites [149][150][151]. Its applications in the sports field are steadily expanding, encompassing enhancements in sports equipment performance and monitoring athletes' physiological indicators.…”
Section: Challenges Of Biomass Waste Graphene In Sports Applicationsmentioning
confidence: 99%
“…Three-dimensional nanostructured graphene not only inherits some unique properties of two-dimensional graphene but also offers numerous novel features, such as a boosted surface area, rapid gas diffusion, and abundant reaction sites [149][150][151]. Its applications in the sports field are steadily expanding, encompassing enhancements in sports equipment performance and monitoring athletes' physiological indicators.…”
Section: Challenges Of Biomass Waste Graphene In Sports Applicationsmentioning
confidence: 99%
“…GO has shown great potential in a variety of fields by virtue of its high surface area [ 88 ], unique mechanical strength [ 89 ], and excellent optical and magnetic properties [ 90 ]. In comparison to other carbon-based nanomaterials, GO is considered a green oxidant, as it is enriched with oxygen-containing functional groups [ 91 , 92 ].…”
Section: Graphene Oxide (Go)mentioning
confidence: 99%
“…[17][18][19][20][21][22] While RGO can potentially overcome fabrication challenges posed by graphene, RGO sheets tend to aggregate, decreasing the surface area exposed to target gases and signicantly decreasing performance in comparison to monolayer graphene or graphene oxide (GO). 22 As an alternative to RGO sheets, nanostructured carbon materials, including porous and foamlike structures, have been recently explored; 14,[22][23][24] however, surfactant-free and simple fabrication of hierarchical graphene structures is still complex. Crumpled graphene oxide (CGO) materials possess a low tendency for aggregation while maintaining high specic surface area and exceptional electronic properties similar to those of at graphene sheets.…”
Section: Introductionmentioning
confidence: 99%