2010
DOI: 10.1088/0022-3727/43/49/495103
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Thickness effect on ultrafast thermalization of carriers in above-band-gap states in ZnO epitaxial films

Abstract: Energy-dependent free-carrier dynamics was investigated in 70 nm (thin) and 1 µm (thick) ZnO epifilms using the optical pump-probe technique. The far-above-band-gap dynamics in the thin epifilm reveals the prolonged relaxation and the slow recovery of renormalized band gap. The band-gap renormalization (BGR) effect is affected by the inefficient carrier-phonon scattering. In addition, the loss of excited carrier density via surface trapping results in an energy-dependent BGR buildup time. However, the far-abov… Show more

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Cited by 17 publications
(11 citation statements)
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“…These results deal with a photogenerated non-equilibrium carriers (electrons and holes). Similar values (1.2 ps, 0.81 ps and 0.69 ps) have been reported earlier [14] for the unspecified photogenerated carrier density. The most recent time-resolved pump-probe optical measurements with the given photogenerated carrier density report slightly shorter relaxation times at higher densities: 0.77 ps [15] and 0.85 ps-0.7 ps [13] (Fig.3, open square and triangle).…”
Section: Discussionsupporting
confidence: 89%
“…These results deal with a photogenerated non-equilibrium carriers (electrons and holes). Similar values (1.2 ps, 0.81 ps and 0.69 ps) have been reported earlier [14] for the unspecified photogenerated carrier density. The most recent time-resolved pump-probe optical measurements with the given photogenerated carrier density report slightly shorter relaxation times at higher densities: 0.77 ps [15] and 0.85 ps-0.7 ps [13] (Fig.3, open square and triangle).…”
Section: Discussionsupporting
confidence: 89%
“…3(a) show non-Markovian fast decay at the beginning but become slower after evolving a certain time. Such phenomena can also be observed in the carrier relaxation in semiconductor materials [35,36].…”
Section: A Non-markovian Decay Regime With No Bound Dsmentioning
confidence: 79%
“…In particular, these semiconductor oxides are good candidates for manufacturing transparent conductive oxides (TCO's) due to its simultaneous high optical transparency and low electrical conductivity. Strong and ultrafast nonlinear optical properties in different zinc oxide (ZnO) structures have been reported [2][3][4][5], and furthermore, ZnO is one of the metal oxide semiconductors more suitable for optoelectronic applications given its non-toxicity and low cost of the raw chemicals [6]. ZnO is an "n-type" wide band gap A II B VI semiconductor with hexagonal wurtzite structure (space group C 4 6v (C6 3 mc)) with lattice parameters of a = 0.3296, and c = 0.52065 nm [7].…”
Section: Introductionmentioning
confidence: 99%