“…In addition, the TAFM experiment was performed under the same conditions in the Ca8.5La1.5(Pt3As8)(Fe2As2)5 single crystal irradiated with protons. For the B//c-axis, both pristine and proton irradiated samples showed magnetic field dependence on the zero-temperature activation energy of U0 ~ B -α , similar to the previously reported results 27 . Interestingly, in proton irradiated samples with more point defects, the magnitude of U0 increased over the entire magnetic field region compared to that in pristine samples.…”
Section: Introductionsupporting
confidence: 90%
“…(4). For the pristine and proton irradiated samples, Compared with iron-based superconductors showing similar Tc, the magnitude of U0(B) in our sample is significantly larger, which means that strong pinning occurred in our sample 27,[36][37][38] . Since the coherence length in the direction perpendicular to the c-axis is about 20 Å, which is about 2.5 times larger than the lattice constants a and b, as discussed above, the normal component region with zero…”
Section: Thermally Activated Flux Motion In the Vortex Liquid Statementioning
confidence: 68%
“…For the study of Tc enhancement as well as the delicate relationship between electronic structure and superconductivity, many experiments such as transport 13,18 , APRES 12,19 , pressure effect 20 , infrared spectroscopy [21][22][23] , upper critical field 11,18,24 , penetration depth 25,26 and thermally activated flux motion (TAFM) 27 have been performed. Recently, TAFM experiments 27 have already been performed for La-doped Ca10-3-8 in the B//c-axis direction up to B=6 T. The result of TAFM analysis for this experiment showed the magnetic field dependence of U0 ~ B -α on the zero-temperature activation energy in the entire measured magnetic field region, which was suggested to be due to the entanglement of vortex lines pinned to the point defect. To understand this more clearly in this paper, we performed TAFM experiments in two directions of B//c-axis and B//ab-plane up to 13 T for Ca8.5La1.5(Pt3As8)(Fe2As2)5 single crystal.…”
To study the difference in the vortex pinning mechanism between in-plane and out-of-plane and the change of these pinning mechanisms due to defects induced by proton irradiation, the in-plane electrical resistivity for pristine and proton irradiated (Ca0.85La0.15)10(Pt3As8)(Fe2As2)5 single crystals in B//c and B//ab up to B = 13 T. Both samples showed a monoclinic crystal structure, which was different from previously known, through crystal structure analysis using the selected area electron diffraction (SAED) method. The protons irradiation incident along the c-axis caused expansion of the lattice constants a and b. The electronic structure changed by the expansion of this lattice constant affected the change of the coherence length ξc significantly shorter than the distance between the superconducting Fe2As2 layers. The vortex in B//ab was mainly pinned by the newly formed normal component with zero Cooper pair due to the short ξc, and ξc increased by proton irradiation reduced the pinning energy. On the other hand, the vortex in B//c was mainly pinned by point defects, and the point defects increased by proton irradiation increased the pinning energy.
“…In addition, the TAFM experiment was performed under the same conditions in the Ca8.5La1.5(Pt3As8)(Fe2As2)5 single crystal irradiated with protons. For the B//c-axis, both pristine and proton irradiated samples showed magnetic field dependence on the zero-temperature activation energy of U0 ~ B -α , similar to the previously reported results 27 . Interestingly, in proton irradiated samples with more point defects, the magnitude of U0 increased over the entire magnetic field region compared to that in pristine samples.…”
Section: Introductionsupporting
confidence: 90%
“…(4). For the pristine and proton irradiated samples, Compared with iron-based superconductors showing similar Tc, the magnitude of U0(B) in our sample is significantly larger, which means that strong pinning occurred in our sample 27,[36][37][38] . Since the coherence length in the direction perpendicular to the c-axis is about 20 Å, which is about 2.5 times larger than the lattice constants a and b, as discussed above, the normal component region with zero…”
Section: Thermally Activated Flux Motion In the Vortex Liquid Statementioning
confidence: 68%
“…For the study of Tc enhancement as well as the delicate relationship between electronic structure and superconductivity, many experiments such as transport 13,18 , APRES 12,19 , pressure effect 20 , infrared spectroscopy [21][22][23] , upper critical field 11,18,24 , penetration depth 25,26 and thermally activated flux motion (TAFM) 27 have been performed. Recently, TAFM experiments 27 have already been performed for La-doped Ca10-3-8 in the B//c-axis direction up to B=6 T. The result of TAFM analysis for this experiment showed the magnetic field dependence of U0 ~ B -α on the zero-temperature activation energy in the entire measured magnetic field region, which was suggested to be due to the entanglement of vortex lines pinned to the point defect. To understand this more clearly in this paper, we performed TAFM experiments in two directions of B//c-axis and B//ab-plane up to 13 T for Ca8.5La1.5(Pt3As8)(Fe2As2)5 single crystal.…”
To study the difference in the vortex pinning mechanism between in-plane and out-of-plane and the change of these pinning mechanisms due to defects induced by proton irradiation, the in-plane electrical resistivity for pristine and proton irradiated (Ca0.85La0.15)10(Pt3As8)(Fe2As2)5 single crystals in B//c and B//ab up to B = 13 T. Both samples showed a monoclinic crystal structure, which was different from previously known, through crystal structure analysis using the selected area electron diffraction (SAED) method. The protons irradiation incident along the c-axis caused expansion of the lattice constants a and b. The electronic structure changed by the expansion of this lattice constant affected the change of the coherence length ξc significantly shorter than the distance between the superconducting Fe2As2 layers. The vortex in B//ab was mainly pinned by the newly formed normal component with zero Cooper pair due to the short ξc, and ξc increased by proton irradiation reduced the pinning energy. On the other hand, the vortex in B//c was mainly pinned by point defects, and the point defects increased by proton irradiation increased the pinning energy.
“…To comprehend the transport properties in Ca10-3-8 and Ca10-4-8 systems, it is necessary to understand: 1, the electronic properties of both the Pt n−δ As 8 and Fe 1−x Pt x As layers, 2, the relationship between T c and variables n, x and δ. In figure 12(a), we plot T c versus total Pt concentration (n-δ+10x) of Ca 10 (Pt n−δ As 8 )((Fe 1−x Pt x ) 2 As 2 ) 5 available in the literature [1][2][3][7][8][9][10][11][12].…”
Superconducting single crystal of Ca10(Pt4As8)((Fe0.92Pt0.08)2As2)5 has been prepared using flux method, and the physical properties of which are careful examined. Resistivity anisotropy between ab plane and c-axis is observed, T-0.5 term originated from the interlayer Josephson coupling is essential to be added to the formula used to describe the out-of-plane resistivity. The density of state (DOS) value at Fermi level derived from the fitting of specific heat data is consistent with the calculation results. Both direct and indirect platinum doping effect have influences on the superconducting transition temperature (Tc) of Ca 10-3(4)-8 system, the Tc of our sample falls well into the trend strip formed by the data reported previously.
“…To study the delicate relationship between electronic structure and superconductivity, various experiments such as transport 1,12 , ARPES 11,13 , upper critical field 10,12,14 , thermally activated vortex pinning 15 , pressure effect 16 , penetration depth 17,18 , infrared spectroscopy experiments [19][20][21] , etc. have already been performed in the Ca10-3-8 family.…”
For newly synthesized hole-doped Ca8.5Na1.5(Pt3As8)(Fe2As2)5 single crystals, we measured the infrared reflectivity spectrum and the magnetic field dependence of magnetoresistivity and Hall resistivity. The results of these two experiments in normal states are well described by two band models. In the normal state below 150 K, the optical conductivity spectrum shows a transfer of spectral weights from the mid-infrared region to the near-infrared region. Meanwhile, the magnetoresistance and Hall resistance show a significant decrease in carrier density at 150 K. These two phenomena are due to the conversion of itinerant electrons to heavy electrons by the strong correlation effect, Hund's coupling. In the superconducting state, the spectral weight in the low frequency region by the superconducting condensate is completely suppressed, which is well analyzed by the generalized Mattis-Bardeen (M-B) model with a two superconducting gap.
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