“…In 1991, Ishida et al [13] reported that the ductility of polycrystalline Ni-Al-based  (B2) alloys is drastically improved by the introduction of the ␥ (A1) phase of Ni solid solution on the grain boundaries of the  phase. Actually, this kind of microstructural control has been attempted in some shape memory alloys, such as Ni-Fe-Al [14,15], Ni-Co-Al [16,17], Ni-Co-Ga [6,18,19] and Ni-Fe-Ga [8,20] alloys, and improvement of ductility has been achieved. For such micrstructural control in two-phase alloys, phase equilibrium information is very important.…”