Abstract:In November 2005 the Guangdong and Hong Kong governments established the Pearl River Delta regional air quality monitoring network ("PRD RAQMN"), which represented the first joint regional air pollution and reporting effort in this rapidly developing and heavy-polluted area in southern China. This project has recorded the air quality trends during the 11 th Five-Year Plan (FYP), implemented between 2006 and 2010, and will continue to do so throughout the period of economic development and stringent emission co… Show more
“…Air quality monitoring data (SO 2 , NO 2 , O 3 , and PM 10 ) were collected from the PRD Regional Air Quality Monitoring Network (Zhong et al, 2013b). The network consists of 16 sites with 13 sites in mainland PRD and 3 sites in Hong Kong, which adequately reflect the spatial patterns of air quality in the PRD region.…”
“…Air quality monitoring data (SO 2 , NO 2 , O 3 , and PM 10 ) were collected from the PRD Regional Air Quality Monitoring Network (Zhong et al, 2013b). The network consists of 16 sites with 13 sites in mainland PRD and 3 sites in Hong Kong, which adequately reflect the spatial patterns of air quality in the PRD region.…”
“…The site was heavily influenced by the intense air pollutant emissions from Guangzhou and Foshan area in spring, autumn and winter (Zhong et al, 2013;Peng et al, 2014).…”
Section: Observation Site and Periodsmentioning
confidence: 99%
“…However, simultaneous on-line measurements of water-soluble ions of PM 2.5 and related precursor gases (HNO 3 , SO 2 and NH 3 ) are still very rare , and seasonal variations of them has not been reported in this region. In this study secondary water-soluble inorganic ions, including SO 4 2-, NO 3 -and NH 4 + in PM 2.5 , and the related gaseous pollutants including HNO 3 , NH 3 , SO 2 and NO 2 were measured simultaneously at a regional atmospheric supersite in the PRD region of Guangdong Province (Zhong et al, 2013) during four different seasons. The goal of this study was to understand the inter-action of the secondary water-soluble ions and their gaseous precursors and thus to reveal the pollution properties of the secondary inorganic ions in the PRD region, providing scientific support for designing effective fine particle pollution control strategies.…”
Based on the online observation of PM 2.5 mass concentration, its water-soluble inorganic ions, and their gaseous precursors during August of 2013 to March of 2014 at the atmospheric supersite in the Pearl River Delta (PRD) region, the inter-action of the secondary compositions and their precursors was discussed, and the pollution properties of the secondary inorganic ions were revealed. During the whole measurement period, the average concentrations of SO 4 2 ) equivalent charge ratio of 1.1. The maximum daily peak concentration of HNO 3 was as high as 18.6 µg m -3 , providing an evidence for the strong oxidizing property of the atmosphere in the PRD region. The theoretical equilibrium constant (K e ) of NH 4 NO 3 is always lower than the observed concentration product (K m = [NH 3 ] × [HNO 3 ]) in spring and winter with higher HNO 3 concentrations; while in over 60% of the time during summer and autumn, mainly during daytime, K e was higher. In general, the strong oxidizing property and NH 3 played important roles in the fine particle pollution in the PRD region.
“…In recent, several measurement studies have also been carried out in China, over which there is an increasing concern of air quality accompanying its fast economic development (e.g., in Lanzhou, Zhang et al, 2009a;Beijing, Liu et al, 2010;Zhang et al, 2011;Xue et al, 2014a). The Pearl River Delta region (PRD) including the adjacent Hong Kong is a hot spot of economic development and air pollution in southern China (Zhong et al, 2013). Previous studies have demonstrated the severity of the photochemical smog problem in this region (Zhang et al, 2007;Zhang et al, 2008;Xue et al, 2014b).…”
Peroxyacetyl nitrate (PAN) is a trace constituent of the atmosphere but plays important roles in air pollution and atmospheric chemistry. To understand the chemical and transport processes of PAN in the Pearl River Delta (PRD) region, measurements of PAN, its precursors and related parameters were made at a regional background site in late summer and late autumn of 2011. Despite the fairly low ambient levels of PAN in general, several photochemical episodes with peak concentrations of PAN and ozone (O 3 ) as high as 4.86 and 189 ppbv were observed when the region was under influence of a tropical cyclone. PAN showed a seasonal variation with higher levels in autumn than in summer. PAN production efficiency, defined as the amount of PAN formed per unit amount of nitrogen oxides (NO x ) oxidized, was examined for the polluted PRD plumes, which indicated that PAN production accounted for on average approximately one third of the NO z formation. The photochemical production efficiency of PAN was much lower with respect to that of O 3 , suggesting that ~2.9 ppbv of PAN could be produced per formation of 100 ppbv of O 3 in the PRD plumes. Varying air masses including maritime air, regional air masses from the PRD, and continental outflow from eastern China were identified, which showed different chemical signatures in terms of both pollution levels and NO z budget. The highest abundances of PAN were measured in the PRD air masses, compared to the lowest concentrations in the marine air. Overall, the present study provides some new insights into the photochemical production and regional transport of PAN in the PRD region, where such investigations were very scarce before.
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