Abstract:Sintering plays a major role in the deactivation of heterogeneous catalysts. However, there is limited understanding of the underlying mechanisms. The two leading mechanisms for sintering are coalescence, the movement of smaller particles migrating along the support and joining other small particles to form larger particles, and Oswald ripening, the movement of adatoms emitted from one particle and by either surface or atmospheric diffusion to join other particles to form larger particles. The rate determining… Show more
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