Low temperature processing of environmentally-friendly (K,Na)NbO 3and CoFe 2 O 4-based layered composites has been accomplished by hot pressing, and their electrical, piezoelectric and magnetoelectric properties have been characterized. High quality composite three-layer CoFe 2 O 4 /K 0.5 Na 0.5 NbO 3 /CoFe 2 O 4 structures with defect-free interfaces have been obtained by hot pressing at only 1000 o C, when highly reactive CoFe 2 O 4 powders obtained by Pechini are used. Negligible chemical reactions at, and interdiffusion across interfaces take place during the low temperature processing, while alkali volatilization is also minimized. Dense, crack-free