The fieldo fc hiral plasmonics has received increasing attention in various areas of nanoscience due to the unprecedented light-matter interactions and promising optical applications. Chiral arrangemento fn anoparticles is one of the strategies employed for fabrication of chiraln anostructures. These arrays exhibit collective chirality,w here the chiroptical properties are governed by the geometricalp arameters with nanometer precision.I nt his regard, the self-assembly of biomolecules, such as peptides, DNA, and macromolecules, and their integration with plasmonic buildingb locks, can provide ar oute for the design and production of chiral plasmonic assemblies. In this Focus Review,w eh ighlight biomolecule-assisted methods for the chiral assembly of plasmonic nanostructures with emphasis on of the types of biomolecules and the geometry of the resulting assemblies. We present an overview of recent achievements in chiral plasmonic assemblies and provide perspectives for future directions in the field of chiral plasmonics.