Abstract:Using symmetry breaking strain to tune the valley occupation of a two-dimensional (2D) electron system in an AlAs quantum well, together with an applied in-plane magnetic field to tune the spin polarization, we independently control the system's valley and spin degrees of freedom and map out a spin-valley phase diagram for the 2D metal-insulator transition. The insulating phase occurs in the quadrant where the system is both spin-and valley-polarized. This observation establishes the equivalent roles of spin a… Show more
“…It is possible that because the UCF noise involves interference between two Feynman propagators, it is more likely to be affected by the localized spins than the WL correction which is determined by a single self intersecting propagator. Note that we have not discussed spatial inhomogeneity or clustering in the distribution of dopants which can lead to coexistence of localized and delocalized phases [14], impact of multiple valleys [39,40], or the inter-site Coulomb interaction [34,35,41] which are unlikely to affect the time reversal symmetry. In summary, magnetoconductivity and noise measurements reveal an unexpected spontaneous breaking of time reversal symmetry in 2D electron systems hosted in atomically confined Si:P and Ge:P crystals.…”
We report experimental evidence of a remarkable spontaneous time reversal symmetry breaking in two dimensional electron systems formed by atomically confined doping of phosphorus (P) atoms inside bulk crystalline silicon (Si) and germanium (Ge). Weak localization corrections to the conductivity and the universal conductance fluctuations were both found to decrease rapidly with decreasing doping in the Si:P and Ge:P δ−layers, suggesting an effect driven by Coulomb interactions. In-plane magnetotransport measurements indicate the presence of intrinsic local spin fluctuations at low doping, providing a microscopic mechanism for spontaneous lifting of the time reversal symmetry. Our experiments suggest the emergence of a new many-body quantum state when two dimensional electrons are confined to narrow half-filled impurity bands.Invariance to time reversal is among the most fundamental and robust symmetries of nonmagnetic quantum systems. Its violation often leads to new and exotic phenomena, particularly in two dimensions (2D), such as the quantized Hall conductance in semiconductor heterostructures [1], the quantum anomalous Hall effect in topological insulators [2] or the predicted chiral superconductivity in graphene [3]. The breaking of time reversal invariance is experimentally achieved either by an external magnetic field or intentional magnetic doping. Here we show that strong Coulomb interactions can also lift the time reversal symmetry in nonmagnetic 2D systems at zero magnetic field.While bulk P-doped Si and Ge have been extensively studied in the context of electron localization in three dimensions [4][5][6][7][8][9], confining the dopants to one or few atomic planes (δ−layers) of the host semiconductor has recently led to a new class of 2D electron system [10][11][12][13]. Electron transport in these atomically confined 2D layers occurs within a 2D impurity band where the effective Coulomb interaction is parameterized in terms of U/γ, with U being the Coulomb energy required to add an additional electron to a dopant site, and γ, the hopping integral between adjacent dopants. Since each dopant P atom contributes one valence electron, the impurity band is intrinsically 'half filled' (schematic in Fig. 1a), which reinforces the interaction effects due to the inbuilt electron-hole symmetry, and forms an ideal platform to explore the rich phenomenology of the 2D MottHubbard model, ranging from Mott metal-insulator transition (MIT) to novel spin excitations and magnetic ordering [14][15][16][17].In this Letter we show evidence of spontaneously broken time reversal symmetry in 2D Si:P and Ge:P δ-layers as the on-site effective Coulomb interaction is increased by decreasing the doping density of P atoms. Quantum transport and noise experiments indicate a strong suppression of quantum interference effects at low doping densities. We could attribute this to a spontaneous breaking of time reversal symmetry which manifest in an unambiguous suppression of universal conductance fluctuations (UCF) at zero magnetic fiel...
“…It is possible that because the UCF noise involves interference between two Feynman propagators, it is more likely to be affected by the localized spins than the WL correction which is determined by a single self intersecting propagator. Note that we have not discussed spatial inhomogeneity or clustering in the distribution of dopants which can lead to coexistence of localized and delocalized phases [14], impact of multiple valleys [39,40], or the inter-site Coulomb interaction [34,35,41] which are unlikely to affect the time reversal symmetry. In summary, magnetoconductivity and noise measurements reveal an unexpected spontaneous breaking of time reversal symmetry in 2D electron systems hosted in atomically confined Si:P and Ge:P crystals.…”
We report experimental evidence of a remarkable spontaneous time reversal symmetry breaking in two dimensional electron systems formed by atomically confined doping of phosphorus (P) atoms inside bulk crystalline silicon (Si) and germanium (Ge). Weak localization corrections to the conductivity and the universal conductance fluctuations were both found to decrease rapidly with decreasing doping in the Si:P and Ge:P δ−layers, suggesting an effect driven by Coulomb interactions. In-plane magnetotransport measurements indicate the presence of intrinsic local spin fluctuations at low doping, providing a microscopic mechanism for spontaneous lifting of the time reversal symmetry. Our experiments suggest the emergence of a new many-body quantum state when two dimensional electrons are confined to narrow half-filled impurity bands.Invariance to time reversal is among the most fundamental and robust symmetries of nonmagnetic quantum systems. Its violation often leads to new and exotic phenomena, particularly in two dimensions (2D), such as the quantized Hall conductance in semiconductor heterostructures [1], the quantum anomalous Hall effect in topological insulators [2] or the predicted chiral superconductivity in graphene [3]. The breaking of time reversal invariance is experimentally achieved either by an external magnetic field or intentional magnetic doping. Here we show that strong Coulomb interactions can also lift the time reversal symmetry in nonmagnetic 2D systems at zero magnetic field.While bulk P-doped Si and Ge have been extensively studied in the context of electron localization in three dimensions [4][5][6][7][8][9], confining the dopants to one or few atomic planes (δ−layers) of the host semiconductor has recently led to a new class of 2D electron system [10][11][12][13]. Electron transport in these atomically confined 2D layers occurs within a 2D impurity band where the effective Coulomb interaction is parameterized in terms of U/γ, with U being the Coulomb energy required to add an additional electron to a dopant site, and γ, the hopping integral between adjacent dopants. Since each dopant P atom contributes one valence electron, the impurity band is intrinsically 'half filled' (schematic in Fig. 1a), which reinforces the interaction effects due to the inbuilt electron-hole symmetry, and forms an ideal platform to explore the rich phenomenology of the 2D MottHubbard model, ranging from Mott metal-insulator transition (MIT) to novel spin excitations and magnetic ordering [14][15][16][17].In this Letter we show evidence of spontaneously broken time reversal symmetry in 2D Si:P and Ge:P δ-layers as the on-site effective Coulomb interaction is increased by decreasing the doping density of P atoms. Quantum transport and noise experiments indicate a strong suppression of quantum interference effects at low doping densities. We could attribute this to a spontaneous breaking of time reversal symmetry which manifest in an unambiguous suppression of universal conductance fluctuations (UCF) at zero magnetic fiel...
“…In the so-called Dirac materials like graphene, two energy bands, corresponding to two equivalent sublattices, intersect linearly at different positions in the momentum space, providing multiple valley degeneracy. Since the valley degeneracy is balanced by crystal symmetry, producing a valley-selective current usually requires breaking crystal symmetry by, e.g., strain [1][2][3]. However, a recent study on a three-dimensional (3D) Dirac material, bismuth, demonstrated that a rotating magnetic field modulates the contribution of each valley to the conduction and also reveals the field-induced valley polarization [7][8][9].…”
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confidence: 99%
“…Controlling the valley degree of freedom can be an effective way to modulate charge conduction and to induce intriguing phases [1][2][3][4][5][6][7][8][9][10]. In the so-called Dirac materials like graphene, two energy bands, corresponding to two equivalent sublattices, intersect linearly at different positions in the momentum space, providing multiple valley degeneracy.…”
We report the valley-selective interlayer conduction of SrMnBi 2 under in-plane magnetic fields. The c-axis resistivity of SrMnBi 2 shows clear angular magnetoresistance oscillations indicating coherent interlayer conduction. Strong fourfold variation of the coherent peak in the c-axis resistivity reveals that the contribution of each Dirac valley is significantly modulated by the in-plane field orientation. This originates from anisotropic Dirac Fermi surfaces with strong disparity in the momentum-dependent interlayer coupling. Furthermore, we found a signature of broken valley symmetry at high magnetic fields. These findings demonstrate that a quasi-two-dimensional anisotropic Dirac system can host a valley-polarized interlayer current through magnetic valley control.
“…This apparent metal insulator transition (MIT) is marked by a "critical carrier density", n c which characterizes the crossover from the higherdensity metallic temperature dependence of the resistivity to the lower-density insulating temperature dependence. For n > n c , the system exhibits a metallic behavior (dρ/dT>0) while for n < n c , the resistivity increases with decreasing temperature and dρ/dT<0 in the insulating phase.In the past twenty years, MIT has been observed in a wide variety of 2D carrier systems such as n-Si MOSFETs [3], n-GaAs [5, 6], p-GaAs [7-9], n-Si/SiGe [10, 11], pSi/SiGe [12, 13] and n-AlAs [14,15]. In the current work we present the first experimental observation of 2D MIT in a narrow gap semiconductor, namely, 2D electrons confined in InAs quantum wells.…”
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confidence: 99%
“…In the past twenty years, MIT has been observed in a wide variety of 2D carrier systems such as n-Si MOSFETs [3], n-GaAs [5, 6], p-GaAs [7-9], n-Si/SiGe [10, 11], pSi/SiGe [12, 13] and n-AlAs [14,15]. In the current work we present the first experimental observation of 2D MIT in a narrow gap semiconductor, namely, 2D electrons confined in InAs quantum wells.…”
We report on the first experimental observation of an apparent metal insulator transition in a 2D electron gas confined in an InAs quantum well. At high densities we find that the carrier mobility is limited by background charged impurities and the temperature dependence of the resistivity shows a metallic behavior with resistivity increasing with increasing temperature. At low densities we find an insulating behavior below a critical density of nc = 5 × 10 10 cm −2 with the resistivity decreasing with increasing temperature. We analyze this transition using a percolation model arising from the failure of screening in random background charged impurities. We also examine the percolation transition experimentally by introducing remote ionized impurities at the surface. Using a bias during cool-down, we modify the screening charge at the surface which strongly affects the critical density. Our study shows that transition from a metallic to an insulating phase in our system is due to percolation transition.The metallic behavior of the resistivity observed at low temperatures in low-disorder two-dimensional (2D) systems is a topic of great interest in condensed matter physics. The scaling theory of localization predicts a noninteracting two-dimensional system in the presence of finite disorder is an insulator at zero temperature in the thermodynamic limit [1]. Indeed early experiments confirmed that in highly-disordered two dimensional electron systems (2DESs) the resistivity shows an insulating logarithmic temperature dependence [2]. The scaling theory was challenged by the observation of an apparent metalinsulator transition in high-mobility electron inversion layers in Si metal-oxide-semiconductor-field-effect transistors (MOSFETs) and later in several other 2D semiconductor systems [3,4]. At higher densities, a metallic temperature dependence of the resistivity, ρ, and a concomitant transition to an insulating phase at lower densities were observed. This apparent metal insulator transition (MIT) is marked by a "critical carrier density", n c which characterizes the crossover from the higherdensity metallic temperature dependence of the resistivity to the lower-density insulating temperature dependence. For n > n c , the system exhibits a metallic behavior (dρ/dT>0) while for n < n c , the resistivity increases with decreasing temperature and dρ/dT<0 in the insulating phase.In the past twenty years, MIT has been observed in a wide variety of 2D carrier systems such as n-Si MOSFETs [3], n-GaAs [5, 6], p-GaAs [7-9], n-Si/SiGe [10, 11], pSi/SiGe [12, 13] and n-AlAs [14,15]. In the current work we present the first experimental observation of 2D MIT in a narrow gap semiconductor, namely, 2D electrons confined in InAs quantum wells. We believe that our work is also the observation of the 2D MIT phenomenon in a material with the lowest value of the dimensionless electron interaction coupling parameter r s (∼ 2). Narrow band-gap materials such as InAs are particularly interesting as they have strong spin-orbit coupling,...
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