1998
DOI: 10.1016/s0030-4018(98)00519-7
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Single-molecule spectroscopy near structured dielectrics

Abstract: We present an analytical approach to the calculation of the linewidth and lineshift of an atom or molecule in the near field of a structured dielectric surface. For soft surface corrugations with amplitude lambda/50, we find variations of the linewidth in the ten percent region. More strikingly, the shift of the molecular resonance can reach several natural linewidths. We demonstrate that the lateral resolution is of the order of the molecule-surface distance. We give a semiquantitative explanation of the outc… Show more

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Cited by 62 publications
(60 citation statements)
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References 41 publications
(73 reference statements)
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“…Note, that this perturbation approach has also been used to study for example the roughness effects for the Casimir force 23,24 . We remark that the perturbation theory can be applied as far as the rms of the surface profiles is the smallest lenght scale of the problem 25 . Then, by inserting the zeroth-order dyadic Green's function from 22 into the expression for the mean transmission coefficient in Eq.…”
Section: A Perturbation Resultsmentioning
confidence: 99%
“…Note, that this perturbation approach has also been used to study for example the roughness effects for the Casimir force 23,24 . We remark that the perturbation theory can be applied as far as the rms of the surface profiles is the smallest lenght scale of the problem 25 . Then, by inserting the zeroth-order dyadic Green's function from 22 into the expression for the mean transmission coefficient in Eq.…”
Section: A Perturbation Resultsmentioning
confidence: 99%
“…Later, atoms in excited energy eigenstates were included in the concept [16]. Effects of surface roughness [17], finite temperature [18] and-in the case of the semi-infinite half space-different materials such as birefringent dielectric [19] and even magnetodielectric matter [20] have been considered.…”
Section: Introductionmentioning
confidence: 99%
“…Later, atoms in excited energy eigenstates were included in the concept [24]. Effects of surface roughness [25] and finite temperature [26,27] and-in the case of the semi-infinite half space-different materials such as birefringent dielectric [28] or even magnetodielectric matter [29] have been studied.…”
Section: Introductionmentioning
confidence: 99%