Construction of Janus-wetting interfaces in solar thermal
evaporation
is one of the most widely applied strategies to overcome salt accumulation
to prolong a system’s lifetime. Nevertheless, hydrophobicity
and steam escape in traditional Janus floating evaporators are negatively
correlated, resulting in the trade-off between salt resistance and
the evaporation rate. Herein, a scalable suspended-slope evaporator
(SSE) based on the inverse wettability polypyrrole (PPy) fabric is
designed to surmount the long-term trade-off for achieving continuous
and stable high-rate water desalination. Experiments and numerical
simulations indicate that the suspended structure opens the “shackles”
brought by the upper hydrophobic PPy fabric to steam escape, and the
Marangoni convection induced by the inclined structure further enhances
salt resistance performance. With this structure employed, SSEs present
good salt tolerance (no obvious salt accumulation in 21 wt % brine
for 5 h) and excellent solar evaporation performance (evaporation
rate of 2.46 kg m–2 h–1 in 3.5
wt % brine, and the energy efficiency is 85.48%). Additionally, there
is no need for special customized high-pressure equipment in the whole
synthesis process, which has great significance for the widespread
practical application. This work elucidates the intrinsic effects
of the device structure on solar evaporators while providing insights
for designing high-efficiency and salt-tolerant solar evaporators.