“…The construction of ordered arrays requires the building block hollow nanoparticles to be uniform in size and shape but has been difficult to achieve. The successful examples of hollow nanoparticle arrays mainly include Si [4], Fe 3 O 4 [5,6], SiO 2 [7], Ni(OH) 2 [8], Au [9,10], Ag [11], TiO 2 and SnO 2 [12], Ni [13,14], and polystyrene [15]. Single-crystalline hollow nanoparticles are expected to have superior properties because of their anisotropic behavior, large surface area, and low material density.…”